Department of Chemistry, Graduate School of Science, Kyoto University, Kyoto 606-8502, Japan.
Philos Trans A Math Phys Eng Sci. 2012 Aug 13;370(1972):3658-71. doi: 10.1098/rsta.2011.0203.
By extending the response function approach developed in nonlinear optics, we analytically derive an expression for the non-Markovianity in the time evolution of a system in contact with a quantum mechanical bath, and find a close connection with the directly observable nonlinear optical response. The result indicates that memory in the bath-induced fluctuations rather than in the dissipation causes non-Markovianity. Initial correlations between states of the system and the bath are shown to be essential for a correct understanding of the non-Markovianity. These correlations are included in our treatment through a preparation function.
通过扩展非线性光学中发展的响应函数方法,我们从分析上推导出了与量子力学浴相互作用的系统随时间演化的非马尔可夫性的表达式,并发现与可直接观测的非线性光学响应有密切的联系。结果表明,是非浴诱导涨落中的记忆而不是耗散引起了非马尔可夫性。系统和浴之间的初始状态相关性对于正确理解非马尔可夫性是至关重要的。我们通过一个准备函数将这些相关性包含在我们的处理中。