Suppr超能文献

二维、三维和四维玻璃形成液体的 Adam-Gibbs 关系。

Adam-Gibbs relation for glass-forming liquids in two, three, and four dimensions.

机构信息

Theoretical Sciences Unit, Jawaharlal Nehru Centre for Advanced Scientific Research, Jakkur Campus, Bangalore 560 064, India.

出版信息

Phys Rev Lett. 2012 Aug 31;109(9):095705. doi: 10.1103/PhysRevLett.109.095705. Epub 2012 Aug 29.

Abstract

The Adam-Gibbs relation between relaxation times and the configurational entropy has been tested extensively for glass formers using experimental data and computer simulation results. Although the form of the relation contains no dependence on the spatial dimensionality in the original formulation, subsequent derivations of the Adam-Gibbs relation allow for such a possibility. We test the Adam-Gibbs relation in two, three, and four spatial dimensions using computer simulations of model glass formers. We find that the relation is valid in three and four dimensions. But in two dimensions, the relation does not hold, and interestingly, no single alternate relation describes the results for the different model systems we study.

摘要

利用实验数据和计算机模拟结果,广泛测试了弛豫时间与构象熵之间的 Adam-Gibbs 关系在玻璃形成体中的适用性。尽管该关系的形式在原始表述中不依赖于空间维度,但 Adam-Gibbs 关系的后续推导允许存在这种可能性。我们使用模型玻璃形成体的计算机模拟在二维、三维和四维空间中测试 Adam-Gibbs 关系。我们发现该关系在三维和四维空间中成立。但是在二维空间中,该关系不成立,有趣的是,没有一个单一的替代关系可以描述我们研究的不同模型系统的结果。

文献AI研究员

20分钟写一篇综述,助力文献阅读效率提升50倍。

立即体验

用中文搜PubMed

大模型驱动的PubMed中文搜索引擎

马上搜索

文档翻译

学术文献翻译模型,支持多种主流文档格式。

立即体验