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金纳米颗粒掺杂聚合物等离子体开关的高效光热激活

Efficient photo-thermal activation of gold nanoparticle-doped polymer plasmonic switches.

作者信息

Weeber J-C, Hassan K, Saviot L, Dereux A, Boissière C, Durupthy O, Chaneac C, Burov E, Pastouret A

机构信息

Laboratoire Interdisciplinaire Carnot de Bourgogne, UMR 6303 CNRS-Université de Bourgogne, Dijon, France.

出版信息

Opt Express. 2012 Dec 3;20(25):27636-49. doi: 10.1364/OE.20.027636.

Abstract

We report on the photo-thermal activation of dielectric loaded plasmonic switches comprised of gold nanoparticle-doped polymer deposited onto a gold film. The plasmonic switches rely on a multi-mode interferometer design and are fabricated by electron beam lithography applied to a positive resin doped with gold nanoparticles at a volume ratio of 0.52%. A cross-bar switching is obtained at telecom wavelengths by pumping the devices with a visible beam having a frequency within the localized surface plasmon resonance band of the embedded nanoparticles. By comparing the switching performances of doped and undoped devices, we show that for the modest doping level we consider, the power needed to activate the doped switches is reduced by a factor 2.5 compared to undoped devices. The minimization of activation power is attributed to enhanced light-heat conversion and optimized spatial heat generation for doped devices and not to a change of the thermo-optic coefficient of the doped polymer.

摘要

我们报道了由沉积在金膜上的金纳米颗粒掺杂聚合物构成的介质加载等离子体开关的光热激活。这些等离子体开关采用多模干涉仪设计,通过电子束光刻技术制造,光刻对象是一种掺杂了体积比为0.52%金纳米颗粒的正性树脂。通过用频率处于嵌入纳米颗粒的局域表面等离子体共振带内的可见光束泵浦这些器件,在电信波长下实现了交叉开关。通过比较掺杂和未掺杂器件的开关性能,我们表明,对于我们所考虑的适度掺杂水平,与未掺杂器件相比,激活掺杂开关所需的功率降低了2.5倍。激活功率的最小化归因于掺杂器件增强的光热转换和优化的空间热生成,而非掺杂聚合物的热光系数的变化。

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