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光热单颗粒卢瑟福散射显微镜。

Photothermal single particle Rutherford scattering microscopy.

机构信息

Molecular Nanophotonics Group, Institute of Experimental Physics I, University of Leipzig, 04103 Leipzig, Germany.

出版信息

Phys Rev Lett. 2013 Mar 8;110(10):103901. doi: 10.1103/PhysRevLett.110.103901. Epub 2013 Mar 6.

Abstract

We demonstrate that the quantum-mechanical description of Rutherford scattering has a photonic counterpart in a new form of single particle photothermal microscopy. Using a split detector we provide experimental evidence that photons are deflected by a photothermal potential that is created by a local refractive index change around a heated nanoparticle. The deflection experienced is shown to be the analog to the deflection of a massive particle wave packet in unscreened spinless Coulomb scattering. The experimentally found focal detection geometry reveals a lateral split feature which will allow new correlation-based velocimetry experiments of absorbing particles with ultrahigh sensitivity.

摘要

我们证明,在一种新形式的单粒子光热显微镜中,卢瑟福散射的量子力学描述有一个光子对应物。通过使用分裂探测器,我们提供了实验证据,表明光子被光热势所偏转,该光热势是由加热纳米颗粒周围的局部折射率变化产生的。所经历的偏折被证明是无屏蔽无自旋库仑散射中大量粒子波包偏折的类似物。实验发现的焦面检测几何形状揭示了一种横向分裂特征,这将允许对具有超高灵敏度的吸收颗粒进行新的基于相关的速度测量实验。

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