Materials and Nano Physics, School of ICT, KTH Royal Institute of Technology, SE-164 40 Kista, Sweden.
Nanotechnology. 2013 Jun 7;24(22):225204. doi: 10.1088/0957-4484/24/22/225204. Epub 2013 May 3.
We measured the exciton lifetime of single silicon quantum dots, fabricated by electron beam lithography, reactive ion etching and oxidation. The observed photoluminescence decays are of mono-exponential character with a large variation (5-45 μs) from dot to dot, even for the same emission energy. We show that this lifetime variation may be the origin of the heavily debated non-exponential (stretched) decays typically observed for ensemble measurements.
我们测量了通过电子束光刻、反应离子刻蚀和氧化工艺制备的单个硅量子点的激子寿命。观察到的光致发光衰减具有单指数特征,即使对于相同的发射能量,不同量子点之间的衰减时间也有很大差异(5-45μs)。我们表明,这种寿命变化可能是通常在集合测量中观察到的强烈争议的非指数(拉伸)衰减的来源。