Institute of Organic Chemistry, RWTH Aachen University, Landoltweg 1, 52074 Aachen (Germany), Fax: (+49) 241-8092391.
Chemistry. 2014 Feb 3;20(6):1691-700. doi: 10.1002/chem.201304331. Epub 2014 Jan 8.
A procedure that enables high yielding access to phosphonic γ-(hydroxyalkyl)butenolides with excellent regio-, diastereo- and enantiocontrol is reported. The simultaneous construction of up to two adjacent quaternary stereogenic centers by a catalytic asymmetric vinylogous Mukaiyama aldol reaction unites biologically and medicinally relevant entities, namely α-hydroxy phosphonates and γ-(hydroxyalkyl)butenolides. This is achieved by utilizing a readily available chiral copper-sulfoximine catalyst showing a broad functional group tolerance for both the electrophilic and nucleophilic reactants. A discussion about potential factors affecting the observed level of enantioselectivity, which stems from the enantiopure sulfoximine ligand, is also included.
本文报道了一种高产的手性膦酸γ-(羟烷基)丁烯内酯的制备方法,该方法具有优异的区域、立体和对映选择性控制。通过催化不对称乙烯基 Mukaiyama 醛醇反应,可以同时构建多达两个相邻的季立体中心,从而将具有生物和医学相关性的实体(即α-羟基膦酸酯和γ-(羟烷基)丁烯内酯)结合在一起。该方法利用了一种易得的手性铜-亚砜亚胺催化剂,该催化剂对亲电和亲核反应物均具有广泛的官能团耐受性。本文还讨论了可能影响观察到的对映选择性水平的因素,这些因素源于手性亚砜亚胺配体。