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基于时域有限差分法的近场等离子体耦合实现连续金属膜结构的稳健多光谱透光性。

Robust multispectral transparency in continuous metal film structures via multiple near-field plasmon coupling by a finite-difference time-domain method.

机构信息

Laboratory of Nanomaterials and Sensors, College of Physics and Communication Electronics, Jiangxi Normal University & Key Laboratory of Optoelectronic and Telecommunication of Jiangxi Province, Nanchang 330022, China.

出版信息

Phys Chem Chem Phys. 2014 Mar 7;16(9):4320-8. doi: 10.1039/c3cp53703j.

Abstract

We propose a robust multispectral transparent plasmonic structure and calculate its transparency response by using the three-dimensional finite-difference time-domain (FDTD) method. The proposed structure is composed of a continuous ultrathin metal film sandwiched by double two-dimensional (2D) hexagonal non-close-packed metal-dielectric multilayer core-shell nanoparticle arrays. The top and bottom plasmonic arrays in such a structure, respectively, act as the light input and output couplers to carry out the efficient trapping and release of light. Near-perfect multispectral optical transparency in the visible and near-infrared regions is achieved theoretically. The calculated electric field distribution patterns show that the near-perfect multispectral optical transparency mainly originates from the excitation and hybridization of shell and core plasmon modes, strong near-field coupling of dipole plasmon modes between adjacent nanoparticles as well as the excitation of surface plasmon waves of the metal film. The robust transparency bands can be efficiently tuned in a large range by varying the structural parameters and the surrounding dielectric environment. The proposed structure also shows additional merits such as a deep sub-wavelength size and fully retained electrical and mechanical properties of the natural metal. These features might provide promising applications in highly integrated optoelectronic devices including plasmonic filters, nanoscale multiplexers, and non-linear optics.

摘要

我们提出了一种稳健的多光谱透明等离子体结构,并通过三维有限差分时域(FDTD)方法计算了其透明响应。所提出的结构由夹在双层二维(2D)非密排金属-介电多层核壳纳米粒子阵列之间的连续超薄金属膜组成。这种结构中的顶部和底部等离子体阵列分别作为光输入和输出耦合器,以实现光的有效捕获和释放。在理论上实现了在可见和近红外区域的近完美多光谱光透明。计算得到的电场分布模式表明,近完美的多光谱光透明性主要源于壳层和核等离子体模式的激发和杂化、相邻纳米粒子之间偶极等离子体模式的强近场耦合以及金属膜表面等离子体波的激发。通过改变结构参数和周围介电环境,可以在很大范围内有效地调节稳健的透明带。所提出的结构还具有其他优点,例如亚波长的深度尺寸以及天然金属的全保留电学和机械性能。这些特性可能为包括等离子体滤波器、纳米级复用器和非线性光学在内的高度集成光电设备提供有前途的应用。

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