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反钙钛矿自旋液体 Tb2Ti2O7 中的磁弹激发。

Magnetoelastic excitations in the pyrochlore spin liquid Tb2Ti2O7.

机构信息

Laboratory for Neutron Scattering, Paul Scherrer Institut, 5232 Villigen PSI, Switzerland.

Laboratory for Developments and Methods, Paul Scherrer Institut, 5232 Villigen PSI, Switzerland.

出版信息

Phys Rev Lett. 2014 Jan 10;112(1):017203. doi: 10.1103/PhysRevLett.112.017203. Epub 2014 Jan 8.

Abstract

At low temperatures, Tb2Ti2O7 enters a spin liquid state, despite expectations of magnetic order and/or a structural distortion. Using neutron scattering, we have discovered that in this spin liquid state an excited crystal field level is coupled to a transverse acoustic phonon, forming a hybrid excitation. Magnetic and phononlike branches with identical dispersion relations can be identified, and the hybridization vanishes in the paramagnetic state. We suggest that Tb2Ti2O7 is aptly named a "magnetoelastic spin liquid" and that the hybridization of the excitations suppresses both magnetic ordering and the structural distortion. The spin liquid phase of Tb2Ti2O7 can now be regarded as a Coulomb phase with propagating bosonic spin excitations.

摘要

在低温下,尽管预期存在磁有序和/或结构变形,但 Tb2Ti2O7 进入自旋液体状态。我们使用中子散射发现,在这种自旋液体状态下,激发的晶体场能级与横向声学声子耦合,形成混合激发。可以识别出具有相同色散关系的磁和类声子支,并且在顺磁态下杂化消失。我们认为 Tb2Ti2O7 恰当地命名为“磁弹性自旋液体”,并且激发的杂化抑制了磁有序和结构变形。现在可以将 Tb2Ti2O7 的自旋液体相视为具有传播玻色子自旋激发的库仑相。

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