Laboratory for Neutron Scattering, Paul Scherrer Institut, 5232 Villigen PSI, Switzerland.
Laboratory for Developments and Methods, Paul Scherrer Institut, 5232 Villigen PSI, Switzerland.
Phys Rev Lett. 2014 Jan 10;112(1):017203. doi: 10.1103/PhysRevLett.112.017203. Epub 2014 Jan 8.
At low temperatures, Tb2Ti2O7 enters a spin liquid state, despite expectations of magnetic order and/or a structural distortion. Using neutron scattering, we have discovered that in this spin liquid state an excited crystal field level is coupled to a transverse acoustic phonon, forming a hybrid excitation. Magnetic and phononlike branches with identical dispersion relations can be identified, and the hybridization vanishes in the paramagnetic state. We suggest that Tb2Ti2O7 is aptly named a "magnetoelastic spin liquid" and that the hybridization of the excitations suppresses both magnetic ordering and the structural distortion. The spin liquid phase of Tb2Ti2O7 can now be regarded as a Coulomb phase with propagating bosonic spin excitations.
在低温下,尽管预期存在磁有序和/或结构变形,但 Tb2Ti2O7 进入自旋液体状态。我们使用中子散射发现,在这种自旋液体状态下,激发的晶体场能级与横向声学声子耦合,形成混合激发。可以识别出具有相同色散关系的磁和类声子支,并且在顺磁态下杂化消失。我们认为 Tb2Ti2O7 恰当地命名为“磁弹性自旋液体”,并且激发的杂化抑制了磁有序和结构变形。现在可以将 Tb2Ti2O7 的自旋液体相视为具有传播玻色子自旋激发的库仑相。