Ecole Polytechnique Fédérale de Lausanne, Institute of Chemical Sciences and Engineering GPAO, Station 6, CH 1015 Lausanne, Switzerland; Institut International d'Ingénierie de l'Eau et de l'Environnement, Laboratoire Eau, Dépollution, Ecosystème et Santé (LEDES), 01 BP 594 Ouagadougou 01, Burkina Faso.
Ecole Polytechnique Fédérale de Lausanne, Institute of Chemical Sciences and Engineering GPAO, Station 6, CH 1015 Lausanne, Switzerland.
Sci Total Environ. 2014 Sep 15;493:229-38. doi: 10.1016/j.scitotenv.2014.05.139. Epub 2014 Jun 17.
The photo-disinfection of water from two different wells (W1, pH: 4.6-5.1 ± 0.02) and (W2 pH: 5.6-5.7 ± 0.02) was carried out during the rainy season at Ouagadougou-Burkina Faso, West Africa. The weather variation during the rainy season significantly affects the photo-disinfection processes (solar disinfection and photo-Fenton). The dilution of the water by rainwater highly affected the chemical composition of the wells' water used in this study; very low iron contents Compared to the ones recorded during the dry season were recorded in all water samples. Both photo-disinfection processes were used to treat 25 L of water in a compound parabolic collector (CPC). None of them have shown the total inactivation of both wild enteric bacteria strains (total coliforms/E. coli and Salmonella spp.) involved in the treatment. However, the total coliforms/E. coli strains were totally inactivated during the exposure under most of the photo-Fenton treatment. Also, the remaining strains, especially those of Salmonella spp. were achieved during the subsequent 24h of dark storage under the action of the Fenton process. Under uniquely solar radiation, total inactivation was recorded only in the total coliforms/E. coli strains. The impact of the available irradiance on the efficiency of the photo-Fenton disinfection of natural water was highlighted during the exposure under high intermittent solar radiation. The impact of the HCO3(-) concentration of both wells' water on the evolution of the pH during the photo-disinfection was recorded. Drastic decrease was noticed after the initial fast increase in presence of low HCO3(-) concentration while a steady state was observed after the increase in presence of higher concentration. The redox activities of the nitrogen components of the water during both photo-disinfection processes have led to increased concentration of nitrite in all the cases and variations were noticed in that of nitrate and ammonia.
在西非布基纳法索的瓦加杜古,对来自两个不同水井(W1,pH:4.6-5.1 ± 0.02)和(W2,pH:5.6-5.7 ± 0.02)的水进行了光消毒。雨季期间的天气变化显著影响了光消毒过程(太阳消毒和光芬顿)。雨水对所研究用水井的水质稀释作用很大,所有水样中的铁含量都非常低,与旱季记录的相比。两种光消毒过程均用于在复合抛物面集热器(CPC)中处理 25 L 的水。在处理过程中,它们都没有完全灭活参与处理的两种野生肠道细菌(总大肠菌群/E. coli 和沙门氏菌属)。然而,在大多数光芬顿处理下,总大肠菌群/E. coli 菌株完全失活。此外,在芬顿过程的后续 24 小时黑暗储存过程中,剩余的菌株,尤其是沙门氏菌属的菌株,也得到了去除。在独特的太阳辐射下,只有在总大肠菌群/E. coli 菌株中才记录到完全失活。在高间歇性太阳辐射下进行暴露时,强调了可用辐照度对天然水的光芬顿消毒效率的影响。记录了两个水井水中 HCO3(-)浓度对光消毒过程中 pH 演变的影响。在低 HCO3(-)浓度存在时,初始快速增加后观察到急剧下降,而在存在更高浓度时,观察到稳定状态。在两种光消毒过程中,水中氮成分的氧化还原活性导致亚硝酸盐浓度增加,硝酸盐和氨的浓度也发生了变化。