Department of Atmospheric Science, University of Washington , 408 ATG Building, Box 351640, Seattle, Washington 98195, United States.
Environ Sci Technol. 2014 Oct 7;48(19):11437-44. doi: 10.1021/es502545k. Epub 2014 Sep 23.
During the summer of 2013, we examined the performance of KCl-coated denuders for measuring gaseous oxidized mercury (GOM) by calibrating with a known source of GOM (i.e., HgBr2) at the North Birmingham SouthEastern Aerosol Research and Characterization (SEARCH) site. We found that KCl-coated denuders have near 95% collection efficiency for HgBr2 in zero air (i.e., air scrubbed of mercury and ozone). However, in ambient air, the efficiency of KCl-coated denuders in capturing HgBr2 dropped to 20-54%. We also found that absolute humidity and ozone each demonstrate a significant inverse correlation with HgBr2 recovery in ambient air. Subsequent laboratory tests with HgBr2 and the KCl-coated denuder show that ozone and absolute humidity cause the release of gaseous elemental Hg from the denuder and thus appear to explain the low recovery in ambient air. Based on these findings, we infer that the KCl denuder method underestimates atmospheric GOM concentrations and a calibration system is needed to accurately measure GOM. The system described in this paper for HgBr2 could be implemented with existing mercury speciation instrumentation and this would improve our knowledge of the response to one potentially important GOM compound.
2013 年夏天,我们通过在北伯明翰东南气溶胶研究和特征(SEARCH)站点用已知的气态氧化汞(GOM)源(即 HgBr2)进行校准,研究了 KCl 涂层沉降器测量 GOM 的性能。我们发现 KCl 涂层沉降器对零气(即经汞和臭氧净化的空气)中的 HgBr2 的收集效率接近 95%。然而,在环境空气中,KCl 涂层沉降器捕获 HgBr2 的效率下降到 20-54%。我们还发现绝对湿度和臭氧都与环境空气中 HgBr2 的回收呈显著负相关。随后用 HgBr2 和 KCl 涂层沉降器进行的实验室测试表明,臭氧和绝对湿度会导致气态元素汞从沉降器中释放出来,因此似乎可以解释环境空气中回收率低的原因。基于这些发现,我们推断 KCl 沉降器法低估了大气 GOM 浓度,需要校准系统来准确测量 GOM。本文中描述的用于 HgBr2 的系统可以与现有的汞形态分析仪器结合使用,这将提高我们对一种潜在重要 GOM 化合物的反应的认识。