Mondal Shrabani, Das Sudip, Baura Alendu, Bag Bidhan Chandra
Department of Chemistry, Visva-Bharati, Santiniketan 731235, India.
J Chem Phys. 2014 Dec 14;141(22):224101. doi: 10.1063/1.4902835.
In this paper, we have studied the properties of a Brownian particle at stationary state in the presence of a fluctuating magnetic field. Time dependence of the field makes the system thermodynamically open. As a signature of that the steady state distribution function becomes function of damping strength, intensity of fluctuations and constant parts of the applied magnetic field. It also depends on the correlation time of the fluctuating magnetic field. Our another observation is that the random magnetic field can induce the resonant activation phenomenon. Here correlation time is increased under the fixed variance of the fluctuating field. But if the correlation time (τ) increases under the fixed field strength then the mean first passage time rapidly grows at low τ and it almost converges at other limit. This is sharp contrast to the usual colored noise driven open system case where the mean first passage time diverges exponentially. We have also observed that a giant enhancement of barrier crossing rate occurs particularly at large strength of constant parts of the applied magnetic field even for very weak fluctuating magnetic field. Finally, break down of the Arrhenius result and disappearance of the Kramers' turn over phenomenon may occur in the presence of a fluctuating magnetic field.
在本文中,我们研究了在波动磁场存在下处于稳态的布朗粒子的性质。磁场的时间依赖性使系统在热力学上成为开放系统。作为其标志,稳态分布函数成为阻尼强度、波动强度和外加磁场恒定部分的函数。它还取决于波动磁场的相关时间。我们的另一个观察结果是,随机磁场可以诱导共振激活现象。这里,在波动场的固定方差下相关时间增加。但是,如果在固定场强下相关时间(τ)增加,那么平均首次穿越时间在低τ时迅速增长,而在其他极限情况下它几乎收敛。这与通常的有色噪声驱动的开放系统情况形成鲜明对比,在后者中平均首次穿越时间呈指数发散。我们还观察到,即使对于非常弱的波动磁场,在外加磁场恒定部分的强度较大时,势垒穿越率也会出现巨大增强。最后,在波动磁场存在的情况下,阿仑尼乌斯结果可能会失效,克莱默斯翻转现象可能会消失。