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放射性同位素光核生产的靶优化

Target optimization for the photonuclear production of radioisotopes.

作者信息

Howard Sean, Starovoitova Valeriia N

机构信息

Idaho State University, Idaho Accelerator Center, 1500 Alvin Ricken Dr, Pocatello, ID 83201, United States.

Idaho State University, Idaho Accelerator Center, 1500 Alvin Ricken Dr, Pocatello, ID 83201, United States.

出版信息

Appl Radiat Isot. 2015 Feb;96:162-167. doi: 10.1016/j.apradiso.2014.12.003. Epub 2014 Dec 5.

Abstract

In this paper we discuss the optimum shape of a target for photonuclear production of radioisotopes using an electron linear accelerator. Different target geometries such as right cylinder, conical frustum, Gaussian volume of revolution and semi-ellipsoid have been considered for the production of (67)Cu via (68)Zn(γ,p)(67)Cu photonuclear reaction. The specific activity (SA) of (67)Cu was simulated for each target shape. Optimum ratio of radius to height for cylindrical targets was found to be between 0.2 and 0.25 for target masses ranging from 20 g to 100 g. It was shown that while some unconventional target shapes, such as semi-elliptical volume of revolution, result in slightly higher specific activities than cylindrical targets, the advantage is not significant and is outweighed by the complexity of the target production and handling. Power deposition into the target was modeled and the trade-off between the maximization of (67)Cu yield and the minimization of target heating has been discussed. The (67)Cu case can easily be extended for production of many other isotopes.

摘要

在本文中,我们讨论了使用电子直线加速器进行放射性同位素光核生产时靶材的最佳形状。为了通过(^{68}Zn(γ,p)^{67}Cu)光核反应生产(^{67}Cu),我们考虑了不同的靶材几何形状,如直圆柱、截头圆锥、高斯旋转体和半椭球体。针对每种靶材形状模拟了(^{67}Cu)的比活度(SA)。对于质量在20克至100克之间的圆柱形靶材,发现半径与高度的最佳比值在0.2至0.25之间。结果表明,虽然一些非常规靶材形状,如半椭球形旋转体,其比活度略高于圆柱形靶材,但这种优势并不显著,且被靶材生产和处理的复杂性所抵消。对靶材中的功率沉积进行了建模,并讨论了(^{67}Cu)产量最大化与靶材加热最小化之间的权衡。(^{67}Cu)的情况可以很容易地扩展到生产许多其他同位素。

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