High Magnetic Field Laboratory, Chinese Academy of Sciences , Hefei 230031 Anhui, People's Republic of China.
Nano Lett. 2015 Feb 11;15(2):869-75. doi: 10.1021/nl503538s. Epub 2015 Jan 16.
Superconductor-insulator transition (SIT) in one-dimensional (1D) nanowires attracts great attention in the past decade and remains an open question since contrasting results were reported in nanowires with different morphologies (i.e., granular, polycrystalline, or amorphous) or environments. Nb2PdS5 is a recently discovered low-dimensional superconductor with typical quasi-1D chain structure. By decreasing the wire diameter in the range of 100-300 nm, we observed a clear SIT with a 1D transport character driven by both the cross-sectional area and external magnetic field. We also found that the upper critical magnetic field (Hc2) decreases with the reduction of nanowire cross-sectional area. The temperature dependence of the resistance below Tc can be described by the thermally activated phase slip (TAPS) theory without any signature of quantum phase slips (QPS). These findings demonstrated that the enhanced Coulomb interactions with the shrinkage of the wire diameter competes with the interchain Josephson-like coupling may play a crucial role on the SIT in quasi-1D system.
一维(1D)纳米线中的超导-绝缘转变(SIT)在过去十年中引起了极大的关注,但由于在具有不同形态(即颗粒状、多晶或非晶)或环境的纳米线中报告了相互矛盾的结果,这个问题仍然没有得到解决。Nb2PdS5 是最近发现的一种具有典型准一维链结构的低维超导体。通过将线径减小到 100-300nm 的范围内,我们观察到了一个明显的 SIT,其具有由横截面积和外部磁场共同驱动的 1D 传输特性。我们还发现,上临界磁场(Hc2)随着纳米线横截面积的减小而减小。在 Tc 以下的电阻温度依赖性可以用热激活相滑移(TAPS)理论来描述,而没有任何量子相滑移(QPS)的特征。这些发现表明,随着线径的缩小,增强的库仑相互作用与类似约瑟夫森的链间耦合竞争可能在准 1D 系统中的 SIT 中起着至关重要的作用。