Zhang Chi, O'Donovan Cathal B, Corwin Eric I, Cardinaux Frédéric, Mason Thomas G, Möbius Matthias E, Scheffold Frank
Department of Physics, University of Fribourg, CH-1700 Fribourg, Switzerland.
School of Physics, Trinity College Dublin, 2, Dublin, Ireland.
Phys Rev E Stat Nonlin Soft Matter Phys. 2015 Mar;91(3):032302. doi: 10.1103/PhysRevE.91.032302. Epub 2015 Mar 2.
We model the packing structure of a marginally jammed bulk ensemble of polydisperse spheres. To this end we expand on the granocentric model [Clusel et al., Nature (London) 460, 611 (2009)], explicitly taking into account rattlers. This leads to a relationship between the characteristic parameters of the packing, such as the mean number of neighbors and the fraction of rattlers, and the radial distribution function g(r). We find excellent agreement between the model predictions for g(r) and packing simulations, as well as experiments on jammed emulsion droplets. The observed quantitative agreement opens the path towards a full structural characterization of jammed particle systems for imaging and scattering experiments.
我们对多分散球体的临界阻塞体系统的堆积结构进行建模。为此,我们在颗粒中心模型[Clusel等人,《自然》(伦敦)460, 611 (2009)]的基础上进行拓展,明确考虑了游离颗粒。这导致了堆积的特征参数(如平均邻居数和游离颗粒分数)与径向分布函数g(r)之间的关系。我们发现g(r)的模型预测与堆积模拟以及阻塞乳液滴实验之间具有极好的一致性。观察到的定量一致性为成像和散射实验中阻塞颗粒系统的完整结构表征开辟了道路。