Mallett B P P, Marsik P, Yazdi-Rizi M, Wolf Th, Böhmer A E, Hardy F, Meingast C, Munzar D, Bernhard C
University of Fribourg, Department of Physics and Fribourg Center for Nanomaterials, Chemin du Musée 3, CH-1700 Fribourg, Switzerland.
Institute of Solid State Physics, Karlsruhe Institute of Technology, Postfach 3640, Karlsruhe 76021, Germany.
Phys Rev Lett. 2015 Jul 10;115(2):027003. doi: 10.1103/PhysRevLett.115.027003. Epub 2015 Jul 8.
With infrared spectroscopy we investigated the spin-reorientation transition from an orthorhombic antiferromagnetic (o-AF) to a tetragonal AF (t-AF) phase and the reentrance of the o-AF phase in the superconducting state of underdoped Ba(1-x)K(x)Fe(2)As(2). In agreement with the predicted transition from a single-Q to a double-Q AF structure, we found that a distinct spin density wave develops in the t-AF phase. The pair breaking peak of this spin density wave acquires much more low-energy spectral weight than the one in the o-AF state which indicates that it competes more strongly with superconductivity. We also observed additional phonon modes in the t-AF phase which likely arise from a Brillouin-zone folding that is induced by the double-Q magnetic structure with two Fe sublattices exhibiting different magnitudes of the magnetic moment.
利用红外光谱,我们研究了欠掺杂的Ba(1 - x)K(x)Fe(2)As(2)在超导态下从正交反铁磁(o - AF)到四方反铁磁(t - AF)相的自旋重取向转变以及o - AF相的再入现象。与从单Q到双Q反铁磁结构的预测转变一致,我们发现t - AF相中出现了明显的自旋密度波。该自旋密度波的对破坏峰比o - AF态中的对破坏峰获得了更多的低能谱权重,这表明它与超导性的竞争更强。我们还在t - AF相中观察到了额外的声子模式,这可能源于由具有两个磁矩大小不同的Fe子晶格的双Q磁结构引起的布里渊区折叠。