Cavendish Laboratory, University of Cambridge, United Kingdom and Department of Applied Mathematics and Theoretical Physics, University of Cambridge, Cambridge CB3 0HE, United Kingdom.
Phys Rev Lett. 2015 Jul 17;115(3):038301. doi: 10.1103/PhysRevLett.115.038301. Epub 2015 Jul 15.
Particle-particle interactions are of paramount importance in every multibody system as they determine the collective behavior and coupling strength. Many well-known interactions such as electrostatic, van der Waals, or screened Coulomb interactions, decay exponentially or with negative powers of the particle spacing r. Similarly, hydrodynamic interactions between particles undergoing Brownian motion decay as 1/r in bulk, and are assumed to decay in small channels. Such interactions are ubiquitous in biological and technological systems. Here we confine two particles undergoing Brownian motion in narrow, microfluidic channels and study their coupling through hydrodynamic interactions. Our experiments show that the hydrodynamic particle-particle interactions are distance independent in these channels. This finding is of fundamental importance for the interpretation of experiments where dense mixtures of particles or molecules diffuse through finite length, water-filled channels or pore networks.
粒子间相互作用在多体系统中至关重要,因为它们决定了系统的集体行为和耦合强度。许多著名的相互作用,如静电、范德华或屏蔽库仑相互作用,随着粒子间距 r 的指数或负幂次而衰减。同样,布朗运动的粒子之间的流体动力学相互作用在整体上以 1/r 的速度衰减,并假定在小通道中衰减。这种相互作用在生物和技术系统中无处不在。在这里,我们将两个处于布朗运动的粒子限制在狭窄的微流道中,并通过流体动力学相互作用来研究它们的耦合。我们的实验表明,在这些通道中,流体动力学的粒子间相互作用与距离无关。这一发现对于解释密集颗粒或分子通过有限长度、充满水的通道或孔隙网络扩散的实验具有重要的基础性意义。