Gallier Stany, Lemaire Elisabeth, Peters François, Lobry Laurent
SAFRAN-Herakles, Le Bouchet Research Center, 91710 Vert le Petit, France.
CNRS-University of Nice, LPMC-UMR 7336, 06108 Nice, France.
Phys Rev E Stat Nonlin Soft Matter Phys. 2015 Aug;92(2):020301. doi: 10.1103/PhysRevE.92.020301. Epub 2015 Aug 21.
Dense suspensions display complex flow properties, intermediate between solid and liquid. When sheared, a suspension self-organizes and forms particle clusters that are likely to percolate, possibly leading to significant changes in the overall behavior. Some theoretical conjectures on percolation in suspensions were proposed by de Gennes some 35 years ago. Although still used, they have not received any validations so far. In this Rapid Communication, we use three-dimensional detailed numerical simulations to understand the formation of percolation clusters and assess de Gennes conjectures. We found that sheared noncolloidal suspensions do show percolation clusters occurring at a critical volume fraction in the range 0.3-0.4 depending on the system size. Percolation clusters are roughly linear, extremely transient, and involve a limited number of particles. We have computed critical exponents and found that clusters can be described reasonably well by standard isotropic percolation theory. The only disagreement with de Gennes concerns the role of percolation clusters on rheology which is found to be weak. Our results eventually validate de Gennes conjectures and demonstrate the relevance of percolation concepts in suspension physics.
稠密悬浮液呈现出介于固体和液体之间的复杂流动特性。受到剪切作用时,悬浮液会自我组织并形成可能发生渗流的颗粒簇,这可能导致整体行为发生显著变化。大约35年前,德热纳提出了一些关于悬浮液中渗流的理论推测。尽管这些推测至今仍在使用,但尚未得到任何验证。在这篇快速通讯中,我们使用三维详细数值模拟来理解渗流簇的形成并评估德热纳的推测。我们发现,受到剪切作用的非胶体悬浮液确实会在0.3至0.4的临界体积分数范围内出现渗流簇,具体数值取决于系统大小。渗流簇大致呈线性,极其短暂,且涉及的颗粒数量有限。我们计算了临界指数,发现这些簇可以用标准的各向同性渗流理论相当好地描述。与德热纳唯一的分歧在于渗流簇在流变学中的作用,我们发现其作用较弱。我们的结果最终验证了德热纳的推测,并证明了渗流概念在悬浮液物理学中的相关性。