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城市环境中金属污染土壤的性质与范围(主题演讲)

Nature and extent of metal-contaminated soils in urban environments (keynote talk).

作者信息

Mielke Howard W

机构信息

Environmental Signaling Laboratory, Department of Pharmacology, Tulane University School of Medicine, New Orleans, LA, USA.

出版信息

Environ Geochem Health. 2016 Aug;38(4):987-99. doi: 10.1007/s10653-016-9792-6. Epub 2016 Jan 11.

Abstract

Research on the nature and extent of metal-contaminated soil began with an urban garden study in Baltimore, MD (USA). Largest quantities of soil metals were clustered in the inner city with lesser amounts scattered throughout metropolitan Baltimore. The probability values of metal clustering varied from P value 10(-15)-10(-23) depending on element. The inner-city clustering of lead (Pb) could not be explained by Pb-based paint alone. A major Pb source was tetraethyl lead (TEL), developed as an anti-knock agent for use in vehicle fuel, thereby making highway traffic flow a toxic substance delivery system in cities. Further study in Minneapolis and St. Paul confirmed the clustering of inner-city soil metals, especially Pb. Based on the evidence, the Minnesota State Legislature petitioned Congress to curtail Pb additives resulting in the rapid phasedown of TEL on January 1, 1986, 10 years ahead of the EPA scheduled ban. Further research in New Orleans, Louisiana (NOLA), verified the link between soil Pb, blood Pb, morbidity, and societal health. Although Pb is a known cause of clinical impairment, there is no known effective medical intervention for reducing children's blood Pb exposure. Ingestion and inhalation are routes of exposure requiring prevention, and soil is a reservoir of Pb. Children's blood Pb exposure observed in pre-Hurricane Katrina (August 29, 2005) NOLA underwent substantial decreases 10 years post-Katrina due to many factors including input of low Pb sediment residues by the storm surge and the introduction of low Pb landscaping materials from outside of the city. Investigation on the topic is ongoing.

摘要

关于金属污染土壤的性质和范围的研究始于美国马里兰州巴尔的摩市的一项城市花园研究。土壤金属含量最高的区域集中在市中心,较少的含量则散布在巴尔的摩大都市地区。金属聚集的概率值因元素而异,范围从P值10(-15)到10(-23)。市中心铅(Pb)的聚集不能仅用含铅涂料来解释。一个主要的铅源是四乙基铅(TEL),它被开发用作车辆燃料的抗爆剂,从而使公路交通流成为城市中的有毒物质输送系统。在明尼阿波利斯和圣保罗的进一步研究证实了市中心土壤金属的聚集,尤其是铅。基于这些证据,明尼苏达州立法机构请求国会减少铅添加剂的使用,导致四乙基铅于1986年1月1日迅速逐步淘汰,比美国环境保护局(EPA)预定的禁令提前了10年。在路易斯安那州新奥尔良市(NOLA)的进一步研究证实了土壤铅、血铅、发病率和社会健康之间的联系。尽管铅是临床损伤的已知原因,但尚无已知有效的医学干预措施来降低儿童的血铅暴露。摄入和吸入是需要预防的暴露途径,而土壤是铅的储存库。在卡特里娜飓风(2005年8月29日)前的新奥尔良市观察到的儿童血铅暴露,在卡特里娜飓风过后10年由于多种因素大幅下降,包括风暴潮带来的低铅沉积物残留以及从城市外部引入的低铅景观材料。对该主题的调查仍在进行中。

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