State Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, No. 390, Qinghe Road, Jiading District, Shanghai 201800, China.
IFSA Collaborative Innovation Center, Shanghai Jiao Tong University, Shanghai 200240, China.
Sci Rep. 2016 May 5;6:25417. doi: 10.1038/srep25417.
A unified picture of femtosecond laser induced precipitation in a cloud chamber is proposed. Among the three principal consequences of filamentation from the point of view of thermodynamics, namely, generation of chemicals, shock waves and thermal air flow motion (due to convection), the last one turns out to be the principal cause. Much of the filament induced chemicals would stick onto the existing background CCN's (Cloud Condensation Nuclei) through collision making the latter more active. Strong mixing of air having a large temperature gradient would result in supersaturation in which the background CCN's would grow efficiently into water/ice/snow. This conclusion was supported by two independent experiments using pure heating or a fan to imitate the laser-induced thermal effect or the strong air flow motion, respectively. Without the assistance of any shock wave and chemical CCN's arising from laser filament, condensation and precipitation occurred. Meanwhile we believe that latent heat release during condensation /precipitation would enhance the air flow for mixing.
提出了一种在云室中飞秒激光诱导沉淀的统一图像。从热力学的角度来看,丝状结构的三个主要后果,即化学物质的产生、冲击波和热气流运动(由于对流),最后一个是主要原因。在丝状结构诱导的许多化学物质会通过碰撞附着在现有的背景 CCN(云凝结核)上,使后者更活跃。具有大温度梯度的空气的强烈混合会导致过饱和度,在过饱和度中,背景 CCN 将有效地生长成水/冰/雪。这一结论得到了两个独立实验的支持,分别使用纯加热或风扇来模拟激光诱导的热效应或强气流运动。在没有任何冲击波和化学 CCN 的情况下,激光细丝产生的冷凝和沉淀发生了。同时,我们相信冷凝/沉淀过程中的潜热释放会增强空气混合的气流。