Taylor A, Keith-Roach M J, Iurian A R, Mabit L, Blake W H
Plymouth University, School of Geography, Earth and Environmental Sciences, Plymouth, PL4 8AA, UK.
Plymouth University, School of Geography, Earth and Environmental Sciences, Plymouth, PL4 8AA, UK; Kemakta Konsult, Stockholm, Sweden.
J Environ Radioact. 2016 Aug;160:80-6. doi: 10.1016/j.jenvrad.2016.04.025. Epub 2016 May 4.
Cosmogenic beryllium-7 has been widely employed as a sediment tracing tool and continued development of its use as a soil erosion tracer requires knowledge of fallout temporal dynamics. Data regarding beryllium-7 fallout in the UK are scarce and here the authors provide a record of beryllium-7 fallout in southwest England spanning a two-year period. A monthly fallout record was developed for Plymouth, UK using regular rainfall sampling to determine beryllium-7 rainfall activity concentration (Bq L(-1)) and deposition flux (Bq m(-2)). Data showed a general tendency for higher activity during the spring/summer months and lower activity in the autumn/winter months. Comparison with data for other UK sites (Chilton and Aberporth) for the same period found significant differences in (7)Be activity in rainwater and lower variability in Plymouth than Chilton and Aberporth. Total deposition was largely controlled by rainfall in Plymouth although regression coefficients suggested greater importance of other atmospheric controls at the Chilton and Aberporth sites. Use of a deposition proportion to rainfall proportion ratio identified periods when deposition was influenced by varying (7)Be activity in rainfall. Broad ranges in ratios were found for Chilton and Aberporth and this has implications for sediment tracer studies requiring estimates of (7)Be deposition flux across months or seasons.
宇宙成因铍 - 7已被广泛用作沉积物示踪工具,而要继续将其开发为土壤侵蚀示踪剂,则需要了解沉降的时间动态。英国关于铍 - 7沉降的数据稀缺,在此作者提供了英格兰西南部为期两年的铍 - 7沉降记录。通过定期采集降雨样本以确定铍 - 7降雨活度浓度(Bq L(-1))和沉积通量(Bq m(-2)),得出了英国普利茅斯的月度沉降记录。数据显示,春夏季的活度总体较高,而秋冬季的活度较低。将同期英国其他站点(奇尔顿和阿伯波特)的数据与之比较发现,雨水中铍 - 7的活度存在显著差异,且普利茅斯的变异性低于奇尔顿和阿伯波特。在普利茅斯,总沉积量在很大程度上受降雨量控制,尽管回归系数表明在奇尔顿和阿伯波特站点其他大气控制因素更为重要。利用沉积比例与降雨比例之比确定了沉积受降雨中铍 - 7活度变化影响的时期。奇尔顿和阿伯波特的比例范围很广,这对需要估算跨月或跨季节铍 - 7沉积通量的沉积物示踪研究有影响。