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评估亚热带垃圾填埋场试验池中的甲烷产生、氧化和排放。

Assessment of methane generation, oxidation, and emission in a subtropical landfill test cell.

机构信息

Centro de Engenharia, Modelagem e Ciências Sociais Aplicadas, Universidade Federal do ABC, Av. dos Estados 5001, Santo André, SP, 09210-580, Brazil.

Departamento de Ciências Biológicas, Universidade Federal de São Paulo, Rua Antônio Doll de Moraes, 105, Diadema, SP, 09920-540, Brazil.

出版信息

Environ Monit Assess. 2016 Aug;188(8):464. doi: 10.1007/s10661-016-5460-7. Epub 2016 Jul 12.

Abstract

This paper presents results of a methane balance assessment in a test cell built in a region with a subtropical climate near São Paulo, Brazil. Measurements and calculations were carried out to obtain the total methane emission to the atmosphere, the methane oxidation rate in the cover, and the total methane generation rate in the test cell. The oxidation rate was obtained through a calculation scheme based on a vertical one-dimensional methane transport in the cover region. The measured maximum and mean methane fluxes to the atmosphere were 124.4 and 15.87 g m(-2) d(-1), respectively. The total methane generation rate obtained for the test cell was 0.0380 ± 0.0075 mol s(-1). The results yielded that 69 % of the emitted methane occurred through the central well and 31 % through the cover interface with the atmosphere. The evaluations of the methane oxidation fraction for localized conditions in the lateral embankment of the test cell yielded 0.36 ± 0.11, while for the whole test cell yielded 0.15 ± 0.10. These results conciliate localized and overall evaluations reported in the literature. The specific methane generation rate obtained for the municipal solid waste with an age of 410 days was 317 ± 62 mol year(-1) ton(-1). This result from the subtropical São Paulo region is lower than reported figures for tropical climates and higher than reported figures for temperate climates.

摘要

本文介绍了在巴西圣保罗附近的亚热带气候地区建造的测试单元中进行的甲烷平衡评估结果。进行了测量和计算,以获得向大气中的总甲烷排放量、覆盖层中的甲烷氧化速率以及测试单元中的总甲烷生成速率。氧化速率是通过基于覆盖区域中垂直一维甲烷传输的计算方案获得的。测量到的最大和平均向大气的甲烷通量分别为 124.4 和 15.87 g m(-2) d(-1)。测试单元获得的总甲烷生成速率为 0.0380 ± 0.0075 mol s(-1)。结果表明,69%的排放甲烷通过中心井发生,31%通过与大气的覆盖层界面发生。对测试单元横向路堤局部条件下的甲烷氧化分数进行评估,得出 0.36 ± 0.11,而对整个测试单元进行评估,得出 0.15 ± 0.10。这些结果调和了文献中报道的局部和整体评估。对于年龄为 410 天的城市固体废物,获得的特定甲烷生成速率为 317 ± 62 mol 年(-1)吨(-1)。来自亚热带圣保罗地区的这一结果低于热带气候地区的报告数据,高于温带气候地区的报告数据。

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