School of Materials Science and Engineering, Dalian University of Technology, Dalian 116024, China.
Soft Matter. 2017 Aug 16;13(32):5409-5420. doi: 10.1039/c7sm00872d.
As a smart soft material, electrorheological elastomers (EREs) present tunable damping capacity and adjustable dynamic moduli on applying an electric field. Most of the previous studies focused on their dynamic moduli, while the damping performance has been neglected. In this study, the damping capacity of two kinds of EREs containing bare TiO and silane coupling agent-modified TiO particles were tested and compared as a function of strain amplitude. The results indicate that the modified TiO particle filled EREs present lower damping capacity when the strain amplitude exceeds 10%, indicating that the interfacial friction between the modified TiO particles and the matrix is decreased due to the stronger interface strength. A theoretical model is developed to describe the damping behaviour of the EREs, which is divided into the intrinsic damping, the interface damping and the electric field induced damping. The experimental results are well matched with the damping curves given by this model under various electric field strengths, and the difference between the damping capacity of the ERE containing bare TiO particles and the one containing modified TiO particles can be mainly ascribed to the effect of weakly and strongly bonded interface damping.
作为一种智能软物质,电流变弹性体(EREs)在施加电场时呈现可调阻尼能力和可调节的动态模量。以前的大多数研究都集中在它们的动态模量上,而阻尼性能则被忽略了。在这项研究中,测试并比较了两种含有裸露 TiO 和硅烷偶联剂改性 TiO 粒子的 EREs 的阻尼能力,作为应变幅度的函数。结果表明,当应变幅度超过 10%时,改性 TiO 粒子填充的 EREs 的阻尼能力较低,这表明由于界面强度增强,改性 TiO 粒子与基体之间的界面摩擦减小。开发了一个理论模型来描述 EREs 的阻尼行为,该模型分为固有阻尼、界面阻尼和电场诱导阻尼。在不同的电场强度下,实验结果与该模型给出的阻尼曲线非常吻合,并且含有裸露 TiO 粒子的 ERE 和含有改性 TiO 粒子的 ERE 的阻尼能力之间的差异主要归因于弱结合界面阻尼和强结合界面阻尼的影响。