Department of Applied Physics (GAP), University of Geneva, 1211 Geneva 4, Switzerland.
Rep Prog Phys. 2018 Feb;81(2):026001. doi: 10.1088/1361-6633/aa8488.
Filamentation of ultra-short TW-class lasers recently opened new perspectives in atmospheric research. Laser filaments are self-sustained light structures of 0.1-1 mm in diameter, spanning over hundreds of meters in length, and producing a low density plasma (10-10 cm) along their path. They stem from the dynamic balance between Kerr self-focusing and defocusing by the self-generated plasma and/or non-linear polarization saturation. While non-linearly propagating in air, these filamentary structures produce a coherent supercontinuum (from 230 nm to 4 µm, for a 800 nm laser wavelength) by self-phase modulation (SPM), which can be used for remote 3D-monitoring of atmospheric components by Lidar (Light Detection and Ranging). However, due to their high intensity (10-10 W cm), they also modify the chemical composition of the air via photo-ionization and photo-dissociation of the molecules and aerosols present in the laser path. These unique properties were recently exploited for investigating the capability of modulating some key atmospheric processes, like lightning from thunderclouds, water vapor condensation, fog formation and dissipation, and light scattering (albedo) from high altitude clouds for radiative forcing management. Here we review recent spectacular advances in this context, achieved both in the laboratory and in the field, reveal their underlying mechanisms, and discuss the applicability of using these new non-linear photonic catalysts for real scale weather control.
超短 TW 类激光的细丝化最近为大气研究开辟了新的视角。激光丝是直径为 0.1-1 毫米、长度跨越数百米的自维持光结构,沿其路径产生低密度等离子体(10-10 cm)。它们源于克尔自聚焦和自生成等离子体或非线性偏振饱和的动态平衡。在空气中非线性传播时,这些丝状结构通过自相位调制(SPM)产生相干超连续谱(对于 800nm 激光波长,从 230nm 到 4μm),可用于通过激光雷达(光探测和测距)远程 3D 监测大气成分。然而,由于其高强度(10-10 W cm),它们还通过激光路径中存在的分子和气溶胶的光致电离和光致解离来改变空气的化学成分。这些独特的特性最近被用于研究调节一些关键大气过程的能力,例如来自雷雨云的闪电、水蒸气凝结、雾的形成和消散以及高空云层的光散射(反照率)以进行辐射强迫管理。在这里,我们回顾了在实验室和野外取得的这方面的最新引人注目的进展,揭示了它们的潜在机制,并讨论了使用这些新的非线性光子催化剂进行实际规模天气控制的适用性。