The Ames Laboratory, US Department of Energy, Iowa State University, Ames, IA, 50011, USA.
Department of Physics and Astronomy, Iowa State University, Ames, IA, 50011, USA.
Nat Commun. 2017 Sep 15;8(1):546. doi: 10.1038/s41467-017-00699-x.
Experimental and theoretical investigations on itinerant ferromagnetic systems under pressure have shown that ferromagnetic quantum criticality is avoided either by a change of the transition order, becoming of the first order at a tricritical point, or by the appearance of modulated magnetic phases. In the first case, the application of a magnetic field reveals a wing-structure phase diagram as seen in itinerant ferromagnets such as ZrZn and UGe. In the second case, no tricritical wings have been observed so far. Here, we report on the discovery of wing-structure as well as the appearance of modulated magnetic phases in the temperature-pressure-magnetic field phase diagram of LaCrGe. Our investigation of LaCrGe reveals a double-wing structure indicating strong similarities with ZrZn and UGe. But, unlike these simpler systems, LaCrGe also shows modulated magnetic phases similar to CeRuPO. This finding provides an example of an additional possibility for the phase diagram of metallic quantum ferromagnets.The study of phase transitions in quantum ferromagnets has shown that the approach to a continuous quantum ferromagnetic transition is typically interrupted by either a tricritical point or a new magnetic phase. Here the authors show that LaCrGe exhibits both these features in its phase diagram.
实验和理论研究表明,在压力下巡游的铁磁系统避免铁磁量子临界点的方式有两种:一种是转变顺序发生变化,在三重临界点变为一级相变;另一种是出现调制磁相。在前一种情况下,施加磁场会揭示出如 ZrZn 和 UGe 等巡游铁磁体中所见到的翼状相图。在后一种情况下,目前尚未观察到三重临界点的翼状结构。在这里,我们报告了在 LaCrGe 的温度-压强-磁场相图中发现的翼状结构以及调制磁相的出现。我们对 LaCrGe 的研究揭示了双翼结构,与 ZrZn 和 UGe 具有很强的相似性。但与这些更简单的系统不同,LaCrGe 还显示出类似于 CeRuPO 的调制磁相。这一发现为金属量子铁磁体的相图提供了另一种可能性。对量子铁磁体相变的研究表明,接近连续量子铁磁转变的过程通常会被三重临界点或新的磁相所中断。在这里,作者表明 LaCrGe 的相图中同时具有这两个特征。