Center for Material Cycles and Waste Management Research, National Institute for Environmental Studies, Onogawa 16-2, Tsukuba, Ibaraki 305-8506, Japan; Department of Risk Management and Environmental Sciences, Yokohama National University Graduate School of Environment and Information Sciences, Tokiwadai 79-1, Hodogaya, Yokohama, Kanagawa 240-8501, Japan.
Center for Material Cycles and Waste Management Research, National Institute for Environmental Studies, Onogawa 16-2, Tsukuba, Ibaraki 305-8506, Japan; Department of Risk Management and Environmental Sciences, Yokohama National University Graduate School of Environment and Information Sciences, Tokiwadai 79-1, Hodogaya, Yokohama, Kanagawa 240-8501, Japan.
J Environ Radioact. 2017 Nov;178-179:290-296. doi: 10.1016/j.jenvrad.2017.08.014. Epub 2017 Sep 19.
Large volumes of decontamination wastes (DW) generated by off-site decontamination activities in Fukushima Prefecture have been incinerated since 2015. The behavior of radioactive cesium during incineration of DW was investigated at a working incineration plant. The incineration discharged bottom ash (BA) and fly ash (FA) with similar levels of radiocesium, and the leachability of the radiocesium from both types of ash was very low (<1%). These results are significantly different from those obtained for the incineration of contaminated municipal solid waste (CMSW) reported in earlier studies. The source of radiocesium in DW-FA is chiefly small particles derived from DW and DW-BA blown into the flue gas, not the deposition of gaseous synthesized radiocesium compounds on the surfaces of ash particles in the flue gas as observed in CMSW incineration. This source difference causes the behavior of radiocesium during waste incineration to differ between DW and CMSW.
自 2015 年以来,福岛县已对场外去污活动产生的大量去污废物(DW)进行了焚烧。在一个工作焚烧厂对 DW 在焚烧过程中的放射性铯行为进行了研究。焚烧产生的底灰(BA)和飞灰(FA)中放射性铯水平相似,两种灰烬中放射性铯的浸出率都非常低(<1%)。这些结果与早期研究中报道的受污染城市固体废物(CMSW)焚烧结果明显不同。DW-FA 中放射性铯的来源主要是来自 DW 和 DW-BA 的小颗粒被吹入烟道气体中,而不是像在 CMSW 焚烧中观察到的气态合成放射性铯化合物在烟道气体中灰颗粒表面的沉积。这种来源差异导致 DW 和 CMSW 废物焚烧过程中放射性铯的行为不同。