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偶极XY反铁磁体Er₂Sn₂O₇中的长程有序

Long-Range Order in the Dipolar XY Antiferromagnet Er_{2}Sn_{2}O_{7}.

作者信息

Petit S, Lhotel E, Damay F, Boutrouille P, Forget A, Colson D

机构信息

Laboratoire Léon Brillouin, CEA, CNRS, Université Paris-Saclay, CE-Saclay, 91191 Gif-sur-Yvette, France.

Institut Néel, CNRS and Université Grenoble Alpes, 38042 Grenoble, France.

出版信息

Phys Rev Lett. 2017 Nov 3;119(18):187202. doi: 10.1103/PhysRevLett.119.187202. Epub 2017 Oct 30.

Abstract

Er_{2}Sn_{2}O_{7} remains a puzzling case among the extensively studied frustrated compounds of the rare-earth pyrochlore family. Indeed, while a first-order transition towards a long-range antiferromagnetic state with the so-called Palmer-Chalker structure is theoretically predicted, it has not yet been observed, leaving the issue as to whether it is a spin-liquid candidate open. We report on neutron scattering and magnetization measurements which evidence a second-order transition towards this Palmer-Chalker ordered state around 108 mK. Extreme care was taken to ensure a proper thermalization of the sample, which has proved to be crucial to successfully observe the magnetic Bragg peaks. At the transition, a gap opens in the excitations, superimposed on a strong quasielastic signal. The exchange parameters, refined from a spin-wave analysis in applied magnetic field, confirm that Er_{2}Sn_{2}O_{7} is a realization of the dipolar XY pyrochlore antiferromagnet. The proximity of competing phases and the strong XY anisotropy of the Er^{3+} magnetic moment might be at the origin of enhanced fluctuations, leading to the unexpected nature of the transition, the low ordering temperature, and the observed multiscale dynamics.

摘要

在稀土焦绿石族经过广泛研究的受挫化合物中,Er₂Sn₂O₇仍然是一个令人困惑的例子。实际上,虽然理论上预测会向具有所谓帕尔默 - 乔克结构的长程反铁磁态发生一级转变,但尚未观察到,这使得它是否是自旋液体候选物的问题仍然悬而未决。我们报告了中子散射和磁化测量结果,这些结果证明在108 mK左右向这种帕尔默 - 乔克有序态发生二级转变。我们极其小心地确保样品的适当热平衡,事实证明这对于成功观察到磁布拉格峰至关重要。在转变时,激发中出现一个能隙,叠加在一个强准弹性信号上。从外加磁场中的自旋波分析中精修得到的交换参数证实,Er₂Sn₂O₇是偶极XY焦绿石反铁磁体的一个实例。竞争相的接近以及Er³⁺磁矩的强XY各向异性可能是增强涨落的根源,导致了转变的意外性质、低有序温度以及观察到的多尺度动力学。

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