Wu Yan-Fei, Zhang Liang, Li Cai-Zhen, Zhang Zhen-Sheng, Liu Song, Liao Zhi-Min, Yu Dapeng
Institute for Quantum Science and Engineering and Department of Physics, South University of Science and Technology of China, Shenzhen, 518055, P. R. China.
Shenzhen Key Laboratory of Quantum Science and Engineering, Shenzhen, 518055, P. R. China.
Adv Mater. 2018 Jul 11:e1707547. doi: 10.1002/adma.201707547.
Dirac semimetal is an emerging class of quantum matters, ranging from 2D category, such as, graphene and surface states of topological insulator to 3D category, for instance, Cd As and Na Bi. As 3D Dirac semimetals typically possess Fermi-arc surface states, the 2D-3D Dirac van der Waals heterostructures should be promising for future electronics. Here, graphene-Cd As heterostructures are fabricated through direct layer-by-layer stacking. The electronic coupling results in a notable interlayer charge transfer, which enables us to modulate the Fermi level of graphene through Cd As . A planar graphene p-n-p junction is achieved by selective modification, which demonstrates quantized conductance plateaus. Moreover, compared with the bare graphene device, the graphene-Cd As hybrid device presents large nonlocal signals near the Dirac point due to the charge transfer from the spin-polarized surface states in the adjacent Cd As . The results enrich the family of van der Waals heterostructure and should inspire more studies on the application of Dirac/Weyl semimetals in spintronics.
狄拉克半金属是一类新兴的量子物质,涵盖从二维范畴(如石墨烯和拓扑绝缘体的表面态)到三维范畴(例如CdAs和NaBi)。由于三维狄拉克半金属通常具有费米弧表面态,二维 - 三维狄拉克范德华异质结构在未来电子学领域应具有广阔前景。在此,通过直接逐层堆叠制备了石墨烯 - CdAs异质结构。电子耦合导致显著的层间电荷转移,这使我们能够通过CdAs调节石墨烯的费米能级。通过选择性修饰实现了平面石墨烯p - n - p结,其展示出量子化的电导平台。此外,与裸石墨烯器件相比,由于相邻CdAs中自旋极化表面态的电荷转移,石墨烯 - CdAs混合器件在狄拉克点附近呈现出大的非局域信号。这些结果丰富了范德华异质结构家族,并应激发更多关于狄拉克/外尔半金属在自旋电子学中应用的研究。