State Key Laboratory of Nuclear Physics and Technology, Peking University, Beijing 100871, People's Republic of China.
Nanotechnology. 2018 Dec 7;29(49):494001. doi: 10.1088/1361-6528/aae189. Epub 2018 Sep 14.
Nanostructured materials have great potential for use as structural materials in advanced nuclear reactors due to the high density of grain boundaries that can serve as sinks to absorb irradiation-induced defects. In the present study, the irradiation tolerance of a La-doped nanocrystalline 304 austenitic stainless steel (NC-La) with a grain size of about 40 nm was investigated under an irradiation of 6 MeV Au ions to 1.5 × 10 ions cm at 600 °C and room temperature. Compared to its coarse-grained counterpart, in La-doped nanocrystalline steel no visible voids were observed at high-temperature irradiation, and no significant difference in extended defects, such as irradiation-induced dislocation loops or clusters, were found between irradiated and unirradiated areas at room temperature irradiation. Furthermore, the nano grain remains stable under irradiation, and no significant grain growth occurs at both irradiation temperatures. The excellent irradiation tolerance of the La-doped nanocrystalline alloys is attributed to the abundant grain boundaries and enhanced stability of nano grains induced by the Zener pinning effect and La segregation on grain boundaries. This study therefore demonstrates the superior irradiation tolerance of the La-doped nanocrystalline steel.
纳米结构材料由于晶界密度高,可作为吸收辐照诱导缺陷的阱,因此在先进核反应堆中用作结构材料具有很大的潜力。本研究在 600°C 和室温下用 6 MeV Au 离子辐照至 1.5×10 离子 cm ,研究了晶粒尺寸约为 40nm 的掺镧纳米晶 304 奥氏体不锈钢(NC-La)的辐照耐受性。与粗晶相比,在高温辐照下,掺镧纳米晶钢中没有观察到明显的空洞,在室温辐照下,辐照区和未辐照区之间也没有发现扩展缺陷(如辐照诱导的位错环或团簇)的明显差异。此外,纳米晶粒在辐照下保持稳定,在两种辐照温度下都没有发生明显的晶粒长大。掺镧纳米晶合金具有优异的辐照耐受性,这归因于晶界的 Zener 钉扎效应和 La 偏析诱导的大量晶界和纳米晶粒稳定性的增强。因此,本研究证明了掺镧纳米晶钢具有优异的辐照耐受性。