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用于γ和α探测的YAG:Ce晶体的生长及闪烁特性

Crystal growth and scintillation properties of YAG:Ce for γ and α detection.

作者信息

Kim MinJeong, Kim H J, Cho J Y, Kaewjaeng S, Kaewkhao J

机构信息

Central Research Institute, Korea Hydro & Nuclear Power Co. Ltd., Daejeon 34101, Republic of Korea.

Department of Physics, Kyungpook National University, Daegu 41566, Reublic of Korea.

出版信息

Appl Radiat Isot. 2019 Mar;145:126-130. doi: 10.1016/j.apradiso.2018.12.011. Epub 2018 Dec 7.

Abstract

A bulk single crystal of yttrium aluminum garnet (YAlO:Ce, YAG:Ce) with good optical quality and free of cracks has been grown successfully by the Kyropoulos method. The dimension of the as grown crystal boule was Ø 20 × 30 cm. The cut and polished crystal sample of dimensions 1 × 1 × 0.5 cm was used for further measurements. The phase purity was confirmed by powder X-ray diffraction pattern analysis. The scintillation properties, such as X-ray emission spectrum, pulse height spectra, energy resolution, and scintillation decay time, were investigated using a Cs γ-ray source. The recorded X-ray emission spectrum shows a broad band between 500 and 700 nm with a peak at around 540 nm, which is attributed to the 5d-4f transition of the Ce ion. The pulse-shape discrimination (PSD) of α and γ signals in a YAG:Ce crystal has been studied by using different pulse shapes. The grown YAG:Ce crystal which is non-hygroscopic, chemically inert, fast inorganic scintillator could be used for radiation detection application in nuclear, and high energy physics.

摘要

采用提拉法成功生长出了光学质量良好且无裂纹的钇铝石榴石(YAlO:Ce,YAG:Ce)块状单晶。生长出的晶体棒尺寸为Ø 20 × 30 cm。尺寸为1 × 1 × 0.5 cm的切割和抛光晶体样品用于进一步测量。通过粉末X射线衍射图谱分析确认了相纯度。使用Cs γ射线源研究了闪烁特性,如X射线发射光谱、脉冲高度谱、能量分辨率和闪烁衰减时间。记录的X射线发射光谱在500至700 nm之间显示出一个宽带,峰值在540 nm左右,这归因于Ce离子的5d - 4f跃迁。通过使用不同的脉冲形状研究了YAG:Ce晶体中α和γ信号的脉冲形状鉴别(PSD)。生长出的YAG:Ce晶体不吸湿、化学惰性、是快速无机闪烁体,可用于核物理和高能物理中的辐射探测应用。

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