Mezei F, Caccamo M T, Migliardo F, Magazù S
European Spallation Source ERIC, Lund, Sweden.
HAS Wigner Research Center, Budapest, Hungary.
J Adv Res. 2019 Feb 16;17:109-116. doi: 10.1016/j.jare.2019.02.003. eCollection 2019 May.
Neutron scattering applications often require discriminating the elastic contribution from the inelastic contribution. For this purpose, correlation spectroscopy offers an effective tool with both pulsed and continuous neutron sources as well as several advantages: the analysis of the neutron velocity distribution can be carried out with a duty factor of 50%, independently on the resolution value; the best statistical accuracy for spectra where the elastic part encompasses most of the integrated intensity is provided. Depending on the statistical chopper position, correlation analysis can be used for both incoming and outgoing neutron velocity determination. Moreover, the correlation technique is very profitable for investigating weak signals in the presence of high background, which is often the case for small samples. To provide instrument flexibility and versatility, an innovative approach comprising tuning resolution by variable Resolution-Elastic Neutron Scattering (RENS) is proposed, offering further benefits by enabling systematic trading of intensity for resolution and vice versa. This study puts into evidence the advantages offered by the use of statistical chopper and of correlation technique for RENS in choosing the best compromise between resolution and beam intensity.
中子散射应用通常需要区分弹性贡献和非弹性贡献。为此,关联光谱学为脉冲和连续中子源提供了一种有效的工具,并且具有多个优点:中子速度分布的分析可以在占空比为50%的情况下进行,与分辨率值无关;对于弹性部分包含大部分积分强度的光谱,能提供最佳统计精度。根据统计斩波器的位置,关联分析可用于确定入射和出射中子速度。此外,关联技术对于在高本底存在的情况下探测微弱信号非常有用,小样品通常就是这种情况。为了提供仪器的灵活性和通用性,提出了一种创新方法,即通过可变分辨率弹性中子散射(RENS)调整分辨率,通过实现强度与分辨率之间的系统权衡,反之亦然,从而带来更多益处。本研究证明了在RENS中使用统计斩波器和关联技术在选择分辨率和束流强度之间的最佳折衷方案时所具有的优势。