Department of Chemical Engineering, College of Petrochemical Technology, Lanzhou University of Technology, Lanzhou, 730050, P. R. China.
ChemSusChem. 2019 Sep 20;12(18):4257-4264. doi: 10.1002/cssc.201901503. Epub 2019 Aug 13.
Solar steam generation by photothermal materials has recently emerged as a new and feasible approach to effectively harvest solar energy in a variety of applications. This work reports an efficient heat localization material based on the renewable cellulose acetate cigarette filters and a reduced graphene oxide coating (RGO-CF) as the light-to-heat conversion layer for solar steam generation. RGO-CF possessed an aligned structure with superhydrophilic nature, lower thermal conductivity (0.0733 Wm K ), and broad light adsorption (≈100 %). These characteristics enable rapid water transportation and excellent light-to-heat conversion by the resulting RGO-CF with an energy conversion efficiency of 94 % under stimulated solar illumination (1 kW m ), which demonstrates that RGO-CF is a promising photothermal conversion material for solar steam generation. Such strategy for preparation of photothermal materials not only reduces the fabrication cost but also provides a fundamental guidance for the practical application of renewable polymer resources from used cigarette filters.
基于可再生醋酸纤维素香烟过滤嘴和还原氧化石墨烯涂层(RGO-CF)的高效热定位材料作为光热转换层用于太阳能蒸汽发生。RGO-CF 具有取向结构和超亲水性质、较低的热导率(0.0733 Wm K )和较宽的光吸收(≈100 %)。这些特性使得 RGO-CF 能够快速输送水,并通过受激太阳光照射(1 kW m )实现出色的光热转换,其能量转换效率为 94 %,表明 RGO-CF 是一种很有前途的用于太阳能蒸汽发生的光热转换材料。这种用于制备光热材料的策略不仅降低了制造成本,还为从废旧香烟过滤嘴中利用可再生聚合物资源提供了实际应用的基础指导。