Satellite-based estimation of hourly PM levels during heavy winter pollution episodes in the Yangtze River Delta, China.

In the developing countries such as China, most well-developed areas have suffered severe haze pollution, which was associated with increased premature morbidity and mortality and attracted widespread public concerns. Since ground-based PM monitoring has limited temporal and spatial coverage, satellite aerosol remote sensing data has been increasingly applied to map large-scale PM characteristics through advanced spatial statistical models. Although most existing research has taken advantage of the polar orbiting satellite instruments, a major limitation of the polar orbiting platform is its limited sampling frequency (e.g., 1-2 times/day), which is insufficient for capturing the PM variability during short but intense heavy haze episodes. As the first attempt, we quantitatively investigated the feasibility of using the aerosol optical depth (AOD) data retrieved by the Geostationary Ocean Color Imager (GOCI) to estimate hourly PM concentrations during winter haze episodes in the Yangtze River Delta (YRD). We developed a three-stage spatial statistical model, using GOCI AOD and fine mode fraction, as well as corresponding monitoring PM concentrations, meteorological and land use data on a 6-km modeling grid with complete coverage in time and space. The 10-fold cross-validation R was 0.72 with a regression slope of 1.01 between observed and predicted hourly PM concentrations. After gap filling, the R value for the three-stage model was 0.68. We further analyzed two representative large regional episodes, i.e., a "multi-process diffusion episode" during December 21-26, 2015 and a "Chinese New Year episode" during February 7-8, 2016. We concluded that AOD retrieved by geostationary satellites could serve as a new valuable data source for analyzing the heavy air pollution episodes.