Center for Correlated Electron Systems, Institute for Basic Science, Seoul, 08826, Korea.
Department of Physics and Astronomy, Seoul National University, Seoul 08826, Korea.
Phys Rev Lett. 2019 Sep 6;123(10):106401. doi: 10.1103/PhysRevLett.123.106401.
Motivated by the novel insulating state of Sr_{2}IrO_{4} from strong spin-orbit coupling (SOC), we investigate, by means of angle resolved photoemission, the metal-insulator transition (MIT) mechanism in Sr_{2-x}La_{x}RhO_{4} whose mother compound is isovalent and isostructural but has smaller SOC strength compared to Sr_{2}IrO_{4}. Transport and angle resolved photoemission results from single crystalline Sr_{2-x}La_{x}RhO_{4} revealed that the MIT occurs coincidentally with a multi- to single-band transition (Lifshitz transition) at x=0.4. Starting from x=0.4, there is a gradual but anomalous enhancement in the band gap size with additional electron doping, suggesting that the insulating phase in Sr_{2-x}La_{x}RhO_{4} is a new type which has been rarely investigated. These results suggest that the insulating phase in Sr_{2-x}La_{x}RhO_{4} is likely induced by the moderate SOC strength and electron doping effect from the La. Our findings not only elucidate the MIT mechanism in Sr_{2-x}La_{x}RhO_{4}, but may also open new avenues for novel MIT research in moderate SOC regimes.
受强自旋轨道耦合 (SOC) 导致 Sr_{2}IrO_{4} 呈现新颖绝缘态的启发,我们通过角分辨光发射研究了母体化合物具有同价同结构但 SOC 强度小于 Sr_{2}IrO_{4} 的 Sr_{2-x}La_{x}RhO_{4} 的金属-绝缘转变 (MIT) 机制。来自 Sr_{2-x}La_{x}RhO_{4} 单晶的输运和角分辨光发射结果表明,MIT 与多能带至单能带转变(Lifshitz 转变)在 x=0.4 时同时发生。从 x=0.4 开始,随着额外电子掺杂,带隙尺寸逐渐但反常地增大,表明 Sr_{2-x}La_{x}RhO_{4} 中的绝缘相是一种很少被研究过的新型相。这些结果表明,Sr_{2-x}La_{x}RhO_{4} 中的绝缘相可能是由中等 SOC 强度和 La 带来的电子掺杂效应诱导的。我们的发现不仅阐明了 Sr_{2-x}La_{x}RhO_{4} 中的 MIT 机制,而且可能为中等 SOC 区新型 MIT 研究开辟新途径。