Hyatt Neil C, Ojovan Michael I
Immobilisation Science Laboratory, Department of Materials Science and Engineering, University of Sheffield, Mappin Street, Sheffield S1 3JD, UK.
Department of Radiochemistry, Lomonosov Moscow State University, Moscow 119991, Russia.
Materials (Basel). 2019 Nov 3;12(21):3611. doi: 10.3390/ma12213611.
Nuclear energy is clean, reliable, and competitive with many useful applications, among which power generation is the most important as it can gradually replace fossil fuels and avoid massive pollution of environment. A by-product resulting from utilization of nuclear energy in both power generation and other applications, such as in medicine, industry, agriculture, and research, is nuclear waste. Safe and effective management of nuclear waste is crucial to ensure sustainable utilization of nuclear energy. Nuclear waste must be processed to make it safe for storage, transportation, and final disposal, which includes its conditioning, so it is immobilized and packaged before storage and disposal. Immobilization of waste radionuclides in durable wasteform materials provides the most important barrier to contribute to the overall performance of any storage and/or disposal system. Materials for nuclear waste immobilization are thus at the core of multibarrier systems of isolation of radioactive waste from environment aimed to ensure long term safety of storage and disposal. This Special Issue analyzes the materials currently used as well as novel materials for nuclear waste immobilization, including technological approaches utilized in nuclear waste conditioning pursuing to ensure efficiency and long-term safety of storage and disposal systems. It focuses on advanced cementitious materials, geopolymers, glasses, glass composite materials, and ceramics developed and used in nuclear waste immobilization, with the performance of such materials of utmost importance. The book outlines recent advances in nuclear wasteform materials including glasses, ceramics, cements, and spent nuclear fuel. It focuses on durability aspects and contains data on performance of nuclear wasteforms as well as expected behavior in a disposal environment.
核能清洁、可靠,且在许多有益应用中具有竞争力,其中发电最为重要,因为它可以逐步替代化石燃料,避免对环境造成大规模污染。核能在发电以及医学、工业、农业和研究等其他应用中产生的副产品是核废料。安全有效地管理核废料对于确保核能的可持续利用至关重要。必须对核废料进行处理,使其在储存、运输和最终处置时安全,这包括对其进行预处理,以便在储存和处置之前将其固定并包装。将废放射性核素固定在耐用的废料形式材料中是对任何储存和/或处置系统的整体性能做出贡献的最重要屏障。因此,用于固定核废料的材料是旨在确保储存和处置长期安全的将放射性废料与环境隔离的多屏障系统的核心。本期特刊分析了目前用于固定核废料的材料以及新型材料,包括在核废料预处理中采用的技术方法,以确保储存和处置系统的效率和长期安全性。它重点关注用于固定核废料的先进胶凝材料、地质聚合物、玻璃、玻璃复合材料和陶瓷,这些材料的性能至关重要。本书概述了核废料形式材料的最新进展,包括玻璃、陶瓷、水泥和乏核燃料。它侧重于耐久性方面,并包含核废料形式的性能数据以及在处置环境中的预期行为。