Institute for Theoretical Physics, Vienna University of Technology, A-1040 Vienna, Austria, EU.
Department of Physics, University of Central Florida, Orlando, Florida 32816, USA.
Phys Rev Lett. 2019 Sep 27;123(13):133203. doi: 10.1103/PhysRevLett.123.133203.
We propose an attosecond extreme ultraviolet pump IR-probe photoionization protocol that employs pairs of counterrotating consecutive harmonics and angularly resolved photoelectron detection, thereby providing a direct measurement of ionization phases. The present method, which we call circular holographic ionization-phase meter, gives also access to the phase of photoemission amplitudes of even-parity continuum states from a single time-delay measurement since the relative phase of one- and two-photon ionization pathways is imprinted in the photoemission anisotropy. The method is illustrated with ab initio simulations of photoionization via autoionizing resonances in helium. The rapid phase excursion in the transition amplitude to both the dipole-allowed (2s2p)^{1}P^{o} and the dipole-forbidden (2p^{2})^{1}D^{e} states are faithfully reproduced.
我们提出了一种阿秒级极紫外泵浦红外探测光致电离协议,该协议采用了两对旋向相反的连续谐波和角度分辨光电子探测,从而提供了对电离相的直接测量。本方法,我们称之为圆全息电离相计,也可以通过单次时间延迟测量获得偶宇称连续态光发射振幅的相位,因为单光子和双光子电离途径的相对相位被记录在光发射各向异性中。该方法通过氦原子自电离共振的从头算模拟进行了说明。对跃迁幅度到偶极允许的(2s2p)^{1}P^{o}和偶极禁戒的(2p^{2})^{1}D^{e}态的快速相移都进行了忠实的再现。