Department of Physics (MC 0435) and Center for Soft Matter and Biological Physics, Robeson Hall, Virginia Tech, Blacksburg, Virginia 24061, USA.
Phys Rev E. 2019 Nov;100(5-1):052210. doi: 10.1103/PhysRevE.100.052210.
We numerically investigate nucleation processes in the transient dynamics of the two-dimensional complex Ginzburg-Landau equation toward its "frozen" state with quasistationary spiral structures. We study the transition kinetics from either the defect turbulence regime or random initial configurations to the frozen state with a well-defined low density of quasistationary topological defects. Nucleation events of spiral structures are monitored using the characteristic length between the emerging shock fronts. We study two distinct situations, namely when the system is quenched either far from the transition limit or near it. In the former deeply quenched case, the average nucleation time for different system sizes is measured over many independent realizations. We employ an extrapolation method as well as a phenomenological formula to account for and eliminate finite-size effects. The nonzero (dimensionless) barrier for the nucleation of single spiral droplets in the extrapolated infinite system size limit suggests that the transition to the frozen state is discontinuous. We also investigate the nucleation of spirals for systems that are quenched close to but beyond the crossover limit and of target waves which emerge if a specific spatial inhomogeneity is introduced. In either of these cases, we observe long, "fat" tails in the distribution of nucleation times, which also supports a discontinuous transition scenario.
我们通过数值研究了二维复金兹堡-朗道方程在向具有准静态螺旋结构的“冻结”状态的瞬态动力学中的成核过程。我们研究了从缺陷湍流区或随机初始构型向具有准静态拓扑缺陷低密度的冻结状态的转变动力学。使用新出现的冲击波之间的特征长度来监测螺旋结构的成核事件。我们研究了两种不同的情况,即当系统远离或靠近相变极限时被淬火。在前者的深淬火情况下,通过多次独立实现测量了不同系统尺寸的平均成核时间。我们采用外推法和唯象公式来解释和消除有限尺寸效应。在扩展的无限系统尺寸极限下,单个螺旋液滴成核的非零(无量纲)势垒表明,向冻结状态的转变是不连续的。我们还研究了在接近但超过交叉点极限的情况下被淬火的系统中螺旋的成核,以及如果引入特定的空间非均匀性,则会出现目标波的情况。在这两种情况下,我们都观察到成核时间分布的长“胖”尾巴,这也支持了不连续转变的情景。