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利用金纳米球增强金纳米板上的 Fano 共振。

Strengthening Fano resonance on gold nanoplates with gold nanospheres.

机构信息

Department of Physics, The Chinese University of Hong Kong, Shatin, Hong Kong SAR, China.

出版信息

Nanoscale. 2020 Jan 23;12(3):1975-1984. doi: 10.1039/c9nr09976j.

Abstract

Plasmonic Fano resonance has attracted extensive attention due to its many applications, including plasmonic sensing, electromagnetically induced transparency, light trapping and stopping, due to its narrow linewidth and asymmetric spectral shape. However, many metal nanostructures are designed with complex geometries to generate Fano resonance and few of them can support a deep Fano dip. Herein we report on the strengthening of the Fano resonance on silicon-supported Au nanoplates through the formation of (Au nanosphere)-(Au nanoplate) heterodimers. The deposition of the Au nanosphere on the top can greatly strengthen the substrate-induced Fano resonance of the Au nanoplate with a deep dip. We also observe that the replacement of the Au nanosphere with a Au nanocube can suppress the excitation of the Fano resonance in the heterodimer. When the sharp corners and edges of the nanocubes gradually become rounded, the Fano resonance appears again with increasing asymmetry. Both the dip depth and wavelength of the Fano resonance can be independently tailored by varying the nanosphere diameter and the nanoplate thickness, respectively. We believe that our results provide an attractive and facile platform for modulating Fano dips and constructing Fano resonance-based devices.

摘要

等离子体激元 Fano 共振由于其在等离子体传感、电磁感应透明、光捕获和停止等方面的许多应用而受到广泛关注,这是由于其窄的线宽和不对称的光谱形状。然而,许多金属纳米结构被设计为具有复杂的几何形状以产生 Fano 共振,其中很少有能够支持深 Fano 陷波。在此,我们通过在硅支撑的 Au 纳米板上形成(Au 纳米球)-(Au 纳米板)杂化二聚体来报告在硅支撑的 Au 纳米板上增强 Fano 共振。Au 纳米球在顶部的沉积可以极大地增强 Au 纳米板的基底诱导 Fano 共振,具有深的陷波。我们还观察到,用 Au 纳米立方体代替 Au 纳米球可以抑制杂二聚体中 Fano 共振的激发。当纳米立方体的尖角和边缘逐渐变圆时,不对称性增加,Fano 共振再次出现。通过改变纳米球的直径和纳米板的厚度,可以分别独立地调整 Fano 共振的陷波深度和波长。我们相信,我们的结果为调制 Fano 陷波和构建基于 Fano 共振的器件提供了一个有吸引力和简便的平台。

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