Gadalla Mena N, Chaudhary Kundan, Zgrabik Christine M, Capasso Federico, Hu Evelyn L
Opt Express. 2020 May 11;28(10):14536-14546. doi: 10.1364/OE.391482.
Titanium nitride (TiN) has been identified as a promising refractory material for high temperature plasmonic applications such as surface plasmon polaritons (SPPs) waveguides, lasers and light sources, and near field optics. Such SPPs are sensitive not only to the highly metallic nature of the TiN, but also to its low loss. We have formed highly metallic, low-loss TiN thin films on MgO substrates to create SPPs with resonances between 775-825 nm. Scanning near-field optical microscopy (SNOM) allowed imaging of the SPP fringes, the accurate determination of the effective wavelength of the SPP modes, and propagation lengths greater than 10 microns. Further, we show the engineering of the band structure of the plasmonic modes in TiN in the mid-IR regime and experimentally demonstrate, for the first time, the ability of TiN to support Spoof Surface Plasmon Polaritons in the mid-IR (6 microns wavelength).
氮化钛(TiN)已被确认为一种有前途的耐火材料,适用于高温等离子体应用,如表面等离子体激元(SPP)波导、激光器和光源以及近场光学。此类表面等离子体激元不仅对氮化钛的高金属性敏感,而且对其低损耗也很敏感。我们已在氧化镁(MgO)衬底上形成了高金属性、低损耗的氮化钛薄膜,以产生共振波长在775 - 825纳米之间的表面等离子体激元。扫描近场光学显微镜(SNOM)能够对表面等离子体激元条纹进行成像,精确测定表面等离子体激元模式的有效波长,并且传播长度大于10微米。此外,我们展示了在中红外波段对氮化钛中等离子体模式能带结构的调控,并首次通过实验证明了氮化钛在中红外(波长6微米)波段支持类表面等离子体激元的能力。