van Nielen Nika, Hentschel Mario, Schilder Nick, Giessen Harald, Polman Albert, Talebi Nahid
Center for Nanophotonics, AMOLF, Science Park 104, 1098 XG Amsterdam, The Netherlands.
4th Physics Institute and Research Center SCoPE, University of Stuttgart, Pfaffenwaldring 57, 70550 Stuttgart, Germany.
Nano Lett. 2020 Aug 12;20(8):5975-5981. doi: 10.1021/acs.nanolett.0c01964. Epub 2020 Jul 17.
Planar electron-driven photon sources have been recently proposed as miniaturized light sources, with prospects for ultrafast conjugate electron-photon microscopy and spectral interferometry. Such sources usually follow the symmetry of the electron-induced polarization: transition-radiation-based sources, for example, only generate p-polarized light. Here we demonstrate that the polarization, the bandwidth, and the directionality of photons can be tailored by utilizing photon-sieve-based structures. We design, fabricate, and characterize self-complementary chiral structures made of holes in an Au film and generate light vortex beams with specified angular momentum orders. The incoming electron interacting with the structure generates chiral surface plasmon polaritons on the structured Au surface that scatter into the far field. The outcoupled radiation interferes with transition radiation creating TE- and TM-polarized Laguerre-Gauss light beams with a chiral intensity distribution. The generated vortex light and its unique spatiotemporal features can form the basis for the generation of structured-light electron-driven photon sources.
平面电子驱动光子源最近被提议作为小型化光源,有望用于超快共轭电子-光子显微镜和光谱干涉测量。此类光源通常遵循电子诱导极化的对称性:例如,基于过渡辐射的光源仅产生p偏振光。在此,我们证明了利用基于光子筛的结构可以调整光子的偏振、带宽和方向性。我们设计、制造并表征了由金膜中的孔构成的自互补手性结构,并产生了具有特定角动量阶数的光涡旋光束。与该结构相互作用的入射电子在结构化金表面产生手性表面等离激元极化子,其散射到远场中。外耦合辐射与过渡辐射相互干涉产生具有手性强度分布的TE和TM偏振拉盖尔-高斯光束。所产生的涡旋光及其独特的时空特性可为结构化光电子驱动光子源的产生奠定基础。