Tsai J-C, Chou M-R, Huang P-C, Fei H-T, Huang J-R
Institute of Physics, Academia Sinica, Taipei, Taiwan.
Soft Matter. 2020 Aug 19;16(32):7535-7543. doi: 10.1039/d0sm00405g.
We study the responses of fluid-immersed soft hydrogel spheres that are sheared under controlled volume fractions. Slippery, deformable particles along with the density-matched interstitial fluid are sandwiched between two opposing rough cones, allowing studies for a wide range of volume fraction φ both above and below the jamming of granular suspension. We utilize sudden cessations of shearing, accompanied by refraction-matched internal imaging, to supplement the conventional flow-curve measurements. At sufficiently high volume fractions, the settling of particles after the cessations exhibits a continuous yet distinct transition over the change of the shear rate. Such changes back out the qualitative difference in the state of flowing prior to the cessations: the quasi-static yielding of a tightly packed network, as opposed to the rapid sliding of particles mediated by the interstitial fluid whose dynamics depends on the driving rate. In addition, we determine the solid-fluid transition using two independent methods: the extrapolation of stress residues and the estimated yield stress from high values of φ, and the settling of particles upon shear cessations as φ goes across the transition. We also verify the power law on values of characteristic stress with respect to the distance from jamming φ - φc, with an exponent close to 2. These results demonstrate a multitude of relaxation timescales behind the dynamics of soft particles, and raise questions on how we extend the existing paradigms of the flow of a densely packed system when the softness is actively involved.
我们研究了在受控体积分数下受到剪切的流体浸没软水凝胶球体的响应。光滑、可变形的颗粒与密度匹配的间隙流体夹在两个相对的粗糙锥体之间,这使得我们能够对颗粒悬浮液堵塞点上下的广泛体积分数φ进行研究。我们利用剪切的突然停止,并辅以折射匹配的内部成像,来补充传统的流动曲线测量。在足够高的体积分数下,停止剪切后颗粒的沉降在剪切速率变化时呈现出连续但明显的转变。这种变化揭示了停止剪切之前流动状态的定性差异:紧密堆积网络的准静态屈服,与间隙流体介导的颗粒快速滑动相反,间隙流体的动力学取决于驱动速率。此外,我们使用两种独立的方法确定固液转变:从高φ值外推应力残余和估计屈服应力,以及当φ跨越转变时剪切停止后颗粒的沉降。我们还验证了特征应力值相对于距堵塞点距离φ - φc的幂律,指数接近2。这些结果证明了软颗粒动力学背后存在多种弛豫时间尺度,并引发了关于当软度积极参与时我们如何扩展现有密集堆积系统流动范式的问题。