State Key Laboratory of Severe Weather & Key Laboratory for Atmospheric Chemistry of China Meteorology Administration, Chinese Academy of Meteorological Sciences, Beijing, 100081, China.
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, 100029, China; Center for Excellence in Urban Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen, 361021, China; University of Chinese Academy of Sciences, Beijing, 100049, China.
Environ Pollut. 2021 Feb 15;271:116325. doi: 10.1016/j.envpol.2020.116325. Epub 2020 Dec 16.
The residual layer (RL) stores a large amount of pollutants, but its effect on near-surface pollution is unknown. In this study, a two-year continuous observation was performed in Beijing using a ceilometer. The generalized boundary layer includes the mixing layer and RL. The results showed that there is no significant seasonal difference in the generalized boundary layer height (GBLH). The average GBLHs in spring, summer, autumn and winter are 1155, 1139, 1036 and 1195 m, respectively. The diurnal variation characteristics of spring, summer and autumn are similar, and the RL disappears when the mixing layer height reaches its peak in the afternoon. In winter, the development of the mixing layer is weak, and there is a 33.8% chance that the RL cannot be breached, thus making the mixing layer height at noon much lower than the GBLH. The concentrations of PM in the mixing layer and RL are 89 and 52 μg m, respectively, and the probability that the PM concentration in the RL was higher than that near the ground was 38.9%. RL transport represents an important beginning of the pollution event during the winter mornings and afternoons in Beijing. This study is helpful to better understand the structure of the RL and its influence on air pollution.
残留层(RL)储存了大量的污染物,但它对近地表污染的影响尚不清楚。本研究在北京进行了为期两年的连续观测,使用了消光仪。广义边界层包括混合层和 RL。结果表明,广义边界层高度(GBLH)没有明显的季节性差异。春季、夏季、秋季和冬季的平均 GBLH 分别为 1155、1139、1036 和 1195 m。春季、夏季和秋季的日变化特征相似,当混合层高度在下午达到峰值时,RL 消失。冬季混合层发展较弱,有 33.8%的可能性 RL 无法突破,从而导致中午混合层高度远低于 GBLH。混合层和 RL 中的 PM 浓度分别为 89 和 52μg/m,RL 中的 PM 浓度高于地面附近的概率为 38.9%。RL 输送代表了北京冬季早晚污染事件的一个重要开端。本研究有助于更好地了解 RL 的结构及其对空气污染的影响。