Wang Yongkai, Wang Qijing, Wang Qianying, Wang Yingying, Li Zhiduo, Lan Xiang, Gao Wei, Han Qingyan, Dong Jun
School of Electronic Engineering, Xi'an University of Posts & Telecommunications, Xi'an 710121 People's Republic of China.
Nanotechnology. 2021 Jul 2;32(38). doi: 10.1088/1361-6528/ac0ac6.
Chiral plasmonic nanostructures have become a promising platform for polarization converters and molecular analysis. However, the circular dichroism (CD) of planar chiral plasmonic nanostructures is always weak and difficult for dynamic adjustment. In this work, graphene sheets (GSs) are introduced in planar metal chiral split rings (MCSRs) to enhance and dynamically adjust their CD effect. The chiral split rings consist of rotated big and small split rings. Simulation results show that the plasmonic coupling between MCSRs and GSs can enhance the absorption and CD spectra of MCSRs at two resonant wavelengths. The surface current distributions reveal that the CD signals are due to the localized surface plasmon resonances on the big and small split rings, respectively. The loss distributions illustrate that the increased loss mainly locates in GSs. In addition, the CD spectra of MCSRs/GSs can be dynamically adjusted and influenced by the Fermi energy of GSs, the geometric parameters of MCSRs and, the mediums in the environment. It can be used to detect the environmental temperature and concentration. The results help to design dynamically adjustable chiral nanostructures and promote their applications in environment detection.
手性等离子体纳米结构已成为用于偏振转换器和分子分析的一个很有前景的平台。然而,平面手性等离子体纳米结构的圆二色性(CD)总是很弱,且难以进行动态调节。在这项工作中,将石墨烯片(GSs)引入平面金属手性裂环(MCSRs)中,以增强并动态调节其CD效应。手性裂环由旋转的大、小裂环组成。模拟结果表明,MCSRs与GSs之间的等离子体耦合可增强MCSRs在两个共振波长处的吸收光谱和CD光谱。表面电流分布表明,CD信号分别归因于大、小裂环上的局域表面等离子体共振。损耗分布表明,增加的损耗主要位于GSs中。此外,MCSRs/GSs的CD光谱可通过GSs的费米能、MCSRs的几何参数以及环境中的介质进行动态调节和影响。它可用于检测环境温度和浓度。这些结果有助于设计动态可调的手性纳米结构,并促进其在环境检测中的应用。