Lin Kang, Chen Xiang, Eckart Sebastian, Jiang Hui, Hartung Alexander, Trabert Daniel, Fehre Kilian, Rist Jonas, Schmidt Lothar Ph H, Schöffler Markus S, Jahnke Till, Kunitski Maksim, He Feng, Dörner Reinhard
Institut für Kernphysik, Goethe-Universität Frankfurt am Main, Frankfurt am Main 60438, Germany.
State Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai 200241, China.
Phys Rev Lett. 2022 Mar 18;128(11):113201. doi: 10.1103/PhysRevLett.128.113201.
The influence of the magnetic component of the driving electromagnetic field is often neglected when investigating light-matter interaction. We show that the magnetic component of the light field plays an important role in nonsequential double ionization, which serves as a powerful tool to investigate electron correlation. We investigate the magnetic-field effects in double ionization of xenon atoms driven by near-infrared ultrashort femtosecond laser pulses and find that the mean forward shift of the electron momentum distribution in light-propagation direction agrees well with the classical prediction, where no under-barrier or recollisional nondipole enhancement is observed. By extending classical trajectory Monte Carlo simulations beyond the dipole approximation, we reveal that double ionization proceeds via recollision-induced doubly excited states, followed by subsequent sequential over-barrier field ionization of the two electrons. In agreement with this model, the binding energies do not lead to an additional nondipole forward shift of the electrons. Our findings provide a new method to study electron correlation by exploiting the effect of the magnetic component of the electromagnetic field.
在研究光与物质相互作用时,驱动电磁场的磁分量的影响常常被忽略。我们表明,光场的磁分量在非顺序双电离中起着重要作用,非顺序双电离是研究电子关联的有力工具。我们研究了由近红外超短飞秒激光脉冲驱动的氙原子双电离中的磁场效应,发现电子动量分布在光传播方向上的平均向前偏移与经典预测吻合良好,其中未观察到势垒下或再碰撞非偶极增强。通过将经典轨迹蒙特卡罗模拟扩展到偶极近似之外,我们揭示了双电离通过再碰撞诱导的双激发态进行,随后是两个电子的后续顺序过势垒场电离。与该模型一致,结合能不会导致电子额外的非偶极向前偏移。我们的发现提供了一种通过利用电磁场磁分量的效应来研究电子关联的新方法。