Han Qingyuan, Zhang Liqun, Wu Youping
State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology Beijing 100029 China
Beijing Engineering Research Centre of Advanced Elastomers, Beijing University of Chemical Technology Beijing 100029 China.
RSC Adv. 2019 Sep 20;9(51):29813-29820. doi: 10.1039/c9ra05833h. eCollection 2019 Sep 18.
In this paper, dynamic fatigue crack propagation properties of natural rubber/silicone rubber (NR/VMQ) composites are studied under constant tearing energy () input. Through dynamic fatigue crack growth testing, it is found that with the increase of VMQ fraction, NR/VMQ exhibits a lower crack growth rate (d/d). The viscoelastic parameters have been recorded in real-time during crack propagation, including the storage modulus ', loss factor tan , and loss compliance modulus '', and their relationships with crack propagation behaviour have been established. The improved crack propagation resistance is attributed to the reduced '', resulting from the synergistic effect of increased ' and decreased tan , and thus more energy dissipation occurred in the linear viscoelastic region in front of the crack tip, which consumed part of the energy for crack growth. Finally, good correlation between d/d and '' could be successfully established.
本文研究了在恒定撕裂能()输入下天然橡胶/硅橡胶(NR/VMQ)复合材料的动态疲劳裂纹扩展特性。通过动态疲劳裂纹扩展试验发现,随着VMQ含量的增加,NR/VMQ复合材料的裂纹扩展速率(d/d)降低。在裂纹扩展过程中实时记录了粘弹性参数,包括储能模量'、损耗因子tan 和损耗柔量'',并建立了它们与裂纹扩展行为的关系。裂纹扩展阻力的提高归因于''的降低,这是由于'增加和tan 降低的协同作用,从而在裂纹尖端前方的线性粘弹性区域发生了更多的能量耗散,消耗了部分裂纹扩展能量。最后,成功建立了d/d与''之间的良好相关性。