Yu Silin, Ni Jingnan, Zhou Zhiling, Xu Shijie, Li Dongting, Li Yong, Qiu Jun
School of Materials Science and Engineering, Tongji University, Shanghai 201804, P. R. China.
School of Physics Science and Engineering, Tongji University, Shanghai 200092, P. R. China.
ACS Appl Mater Interfaces. 2022 Jun 22;14(24):28145-28153. doi: 10.1021/acsami.2c01599. Epub 2022 Jun 7.
Noise is a threat to human life quality and an invisible killer that causes many chronic diseases. The vast majority of porous sound absorbers are single-phased, which limits their sound absorption potential. Herein, a graphene-decorated porous system (GDPS) prepared using the immersion-hydrothermal-freezing self-assembly method is reported as an efficient sound absorber based on its unique consecutive double three-dimensional (dual-3D) structure. Due to the increased tortuosity and other gain effects, the novel structure can achieve the perfect broadband absorption at a wide bandwidth in which the sound absorption coefficient exceeds 0.9 easily. Within the effective thicknesses, the widest perfect absorption bandwidth of 814-6400 Hz is realized. Moreover, a higher graphene concentration and the addition of a polymer are found to be able to decrease the absorption frequency to the lowest values of 1979 and 1544 Hz, respectively. The design of a unique dual-3D structure opens up new strategies and applications to use graphene aerogels in noise and vibration applications.
噪声是对人类生活质量的一种威胁,是导致许多慢性疾病的无形杀手。绝大多数多孔吸声器是单相的,这限制了它们的吸声潜力。在此,报道了一种基于独特的连续双三维(双3D)结构,采用浸渍-水热-冷冻自组装法制备的石墨烯修饰多孔系统(GDPS)作为一种高效吸声器。由于曲折度增加和其他增益效应,这种新型结构能够在很宽的带宽内实现完美的宽带吸收,其中吸声系数很容易超过0.9。在有效厚度范围内,实现了814-6400Hz的最宽完美吸收带宽。此外,发现较高的石墨烯浓度和添加聚合物能够分别将吸收频率降低到1979Hz和1544Hz的最低值。独特的双3D结构设计为石墨烯气凝胶在噪声和振动应用中开辟了新的策略和应用。