Lin Bo-Yen, Li Yi-Ru, Chen Chia-Hsuan, Hsu Hao-Chun, Wei Mao-Kuo, Lee Jiun-Haw, Chiu Tien-Lung
Opt Express. 2022 May 23;30(11):18066-18078. doi: 10.1364/OE.449065.
This study reported the effects of electron transport layer (ETL) thickness on light extraction in corrugated organic light-emitting diodes (OLEDs) and each layer in OLEDs exhibited a periodical corrugated structure, which was determined by depositing thin films on a glass substrate with a nanoimprinted blazed grating structure. The insight is that light extraction in corrugated OLEDs significantly depends on the ETL thickness. Varying the ETL thickness changed the distribution of carrier recombination and led to exciton formation and optical interference, thereby resulting in different attribution of optical loss modes in OLEDs, which increased or even decreased light extraction and device efficiency. Trapped light extraction from the surface plasmon polariton (SPP) and waveguide (WG) modes was identified by splitting the light into transverse electric and transverse magnetic emissions. Thus, the contributions from the individual SPP and WG modes to the external quantum efficiency (EQE) were distinctly clarified by comparing the experimental results with the theoretical calculations. At the ETL thickness of 115 nm, the corrugated OLED exhibited a significantly enhanced (1.83-fold) EQE compared to the planar one due to the effective extraction of trapped light from the SPP and WG modes. The EQE was enhanced by 0.5%, wherein 0.39% came from the WG mode and 0.11% came from the SPP mode.
本研究报道了电子传输层(ETL)厚度对波纹状有机发光二极管(OLED)光提取的影响,OLED中的每一层都呈现出周期性的波纹结构,该结构是通过在具有纳米压印闪耀光栅结构的玻璃基板上沉积薄膜来确定的。关键在于,波纹状OLED中的光提取显著取决于ETL厚度。改变ETL厚度会改变载流子复合的分布,并导致激子形成和光干涉,从而导致OLED中光损耗模式的不同归因,这会增加甚至降低光提取和器件效率。通过将光分离为横向电和横向磁发射,识别出了表面等离激元极化激元(SPP)和波导(WG)模式的陷获光提取。因此,通过将实验结果与理论计算进行比较,明确地阐明了各个SPP和WG模式对外部量子效率(EQE)的贡献。在ETL厚度为115 nm时,由于有效地从SPP和WG模式中提取了陷获光,波纹状OLED与平面OLED相比,其EQE显著提高(1.83倍)。EQE提高了0.5%,其中0.39%来自WG模式,0.11%来自SPP模式。