Che Kai, Chen Chong-Ming, Zheng Qing-Yu, Fan Hui, Wei Ming-Lei, Luo Peng, Yu Jin-Xing
State Grid Hebei Electric Power Research Institute, Shijiazhuang 050021, China.
Norendar International LTD., Shijiazhuang 050011, China.
Huan Jing Ke Xue. 2022 Oct 8;43(10):4578-4589. doi: 10.13227/j.hjkx.202201032.
The aim of this study was to reveal the influence of heavy metal emissions from the flue gas of coal-fired power plants on the surrounding soil environment. Seven heavy metals, including As, Cd, Cr, Cu, Pb, Hg, and Ni, were detected in the flue gas of six coal-fired power plants in Shijiazhuang, and the heavy metals in the soil surrounding the power plants were analyzed. The source analysis and health risk assessment of the heavy metals were carried out. The results showed that after a series of flue gas pollutant control measures, the emission concentrations of different heavy metals in the flue gas of the coal-fired power plants ranged from 0.11 to 6.32 mg·(MW·h), and Cu, Cr, and Ni were the main pollutants. The total amount of the seven heavy metal elements discharged into the atmosphere by each power plant was 33.56-275.71 kg·a. The average contents of Cr, Cu, Pb, Hg, and Ni in the surface soil surrounding the coal-fired power plant were higher than the background values of Hebei soil, and the contents were 1.16-2.32 times higher than the background values. The heavy metal content in the soil around the power plants was proportional to the heavy metal emissions in the flue gas. The heavy metal content in the soil under different wind directions first increased and then decreased gradually with the increase in distance from the power plants. Source analysis showed that coal combustion emissions contributed the most to heavy metals in soil around the power plants (41.4%), followed by industrial emissions (23.6%) and transportation emissions (19.6%). Altogether, human activities played a leading role in soil heavy metal enrichment, accounting for 84.6%. The health risk assessment showed that the overall health risk of metal elements in the soil surrounding the power plant was within acceptable limits.
本研究旨在揭示燃煤电厂烟气中重金属排放对周边土壤环境的影响。对石家庄市6家燃煤电厂烟气中的砷(As)、镉(Cd)、铬(Cr)、铜(Cu)、铅(Pb)、汞(Hg)和镍(Ni)7种重金属进行了检测,并对电厂周边土壤中的重金属进行了分析。开展了重金属的源分析和健康风险评估。结果表明,经过一系列烟气污染物控制措施后,燃煤电厂烟气中不同重金属的排放浓度为0.11~6.32 mg·(MW·h),主要污染物为铜、铬和镍。各电厂排入大气的7种重金属元素总量为33.56~275.71 kg·a。燃煤电厂周边表层土壤中铬、铜、铅、汞和镍的平均含量高于河北土壤背景值,含量比背景值高1.16~2.32倍。电厂周边土壤中的重金属含量与烟气中的重金属排放量成正比。不同风向土壤中的重金属含量随着距电厂距离的增加先升高后逐渐降低。源分析表明,燃煤排放对电厂周边土壤重金属的贡献最大(41.4%),其次是工业排放(23.6%)和交通排放(19.6%)。总体而言,人类活动在土壤重金属富集过程中起主导作用,占84.6%。健康风险评估表明,电厂周边土壤中金属元素的总体健康风险在可接受范围内。