Opt Express. 2022 Aug 15;30(17):30394-30404. doi: 10.1364/OE.464798.
Chiral metamaterials with circular dichroism (CD) or asymmetric transmission (AT) draw enormous attention for their attractive applications in polarization transformers, circular polarizers, and biosensing. In this study, a feasible trilayer chiral metamaterials (TCM) is designed and investigated in theory and simulation. The proposed TCM is composed of a nanoslit layer and a Babinet-complementary nanorod layer separated by a nanoslit spacer. Owing to symmetry breaking by the tilted nanoslit in metal film, the TCM shows simultaneous CD and AT effects in the near-infrared region. The simulated electric charge distributions prove that the chirality arises from the excitation of asymmetric electric dipole resonant modes due to the coupling of adjacent unit cells. Moreover, CD and AT can be tuned by the tilted angle of the nanoslit and the thickness of the spacer, the fitting functions of which are consistent with the theoretical formulas based on transmittance matrix analysis. The proposed nanostructure offers a potential strategy for manipulating metamaterials with simultaneous CD and AT effects, allowing a multitude of exciting applications such as ultra-sensitive polarization transformer and biosensor.
手性超材料具有圆二色性 (CD) 或不对称传输 (AT),在偏振转换器、圆偏振器和生物传感等方面具有吸引力,因此受到了极大的关注。在本研究中,我们从理论和模拟两个方面设计并研究了一种可行的三层手性超材料 (TCM)。所提出的 TCM 由纳米狭缝层和巴宾内互补纳米棒层组成,中间由纳米狭缝间隔层隔开。由于金属膜中倾斜纳米狭缝引起的对称性破坏,TCM 在近红外区域表现出同时具有 CD 和 AT 效应。模拟的电荷分布证明,手性源于由于相邻单元之间的耦合而激发的不对称电偶极共振模式。此外,CD 和 AT 可以通过纳米狭缝的倾斜角和间隔层的厚度来调节,其拟合函数与基于透射率矩阵分析的理论公式一致。所提出的纳米结构为同时具有 CD 和 AT 效应的超材料的操控提供了一种潜在策略,为超灵敏偏振转换器和生物传感器等多种令人兴奋的应用开辟了道路。