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在准自由支撑极限下薄金属膜中的近最大微波吸收。

Near-maximum microwave absorption in a thin metal film at the pseudo-free-standing limit.

作者信息

Haddadi M Mahsa, Das Bamadev, Jeong Jeeyoon, Kim Sunghwan, Kim Dai-Sik

机构信息

Department of Physics and Quantum Photonics Institute, Ulsan National Institute of Science and Technology (UNIST), Ulsan, 44919, Republic of Korea.

Department of Physics, Institute of Quantum Convergence Technology, Kangwon National University, 1 Gangwondaehak-gil, Chuncheon-si, 24341, Gangwon-do, Republic of Korea.

出版信息

Sci Rep. 2022 Nov 1;12(1):18386. doi: 10.1038/s41598-022-23119-7.

Abstract

Electromagnetic absorbers based on ultra-thin metallic film are desirable for many applications such as plasmonics, metamaterials, and long-wavelength detectors. A metallic film will achieve a maximum 50% of electromagnetic wave absorption, frequency independent, at a thickness defined by its conductivity, typically in the sub-Angstrom range for good metals if bulk conductivity is maintained throughout. This makes it extremely difficult to obtain substantial absorption from thin metal films, in contrast to 2D materials such as graphene. Luckily, however, from a practical point of view, metal conductivity is drastically reduced as the film becomes sub-100 nm, to make it a race between the thinnest possible metal thickness experimentally achievable vs the conductivity reduction. Here, we demonstrate a near-50% absorption at a gold film thickness of 6.5 nm, with conductivity much reduced from the bulk value, down to the range of 10 Siemens per meter. Studying the effect of the substrate thickness, we found that the common cover glass, with its thickness much smaller than the wavelength, achieves symmetric absorption of 44%, implying that a pseudo-free-standing limit is achieved. Our work may find applications in infrared sensing as in bolometers and biomedical sensing using microwaves.

摘要

基于超薄金属膜的电磁吸收器在诸如等离子体学、超材料和长波长探测器等许多应用中都很有需求。金属膜在由其电导率定义的厚度下,将实现与频率无关的最大50%的电磁波吸收,对于良金属而言,如果整体电导率始终保持,该厚度通常在亚埃范围内。这使得从薄金属膜中获得大量吸收极其困难,这与二维材料(如石墨烯)形成对比。然而,幸运的是,从实际角度来看,当金属膜厚度小于100纳米时,其电导率会急剧降低,这使得在实验上可实现的尽可能薄的金属厚度与电导率降低之间形成了一场竞赛。在此,我们展示了在金膜厚度为6.5纳米时接近50%的吸收率,此时电导率比体值大幅降低,降至每米10西门子的范围。通过研究衬底厚度的影响,我们发现普通盖玻片,其厚度远小于波长,实现了44%的对称吸收,这意味着达到了一种准自由站立极限。我们的工作可能在红外传感(如测辐射热计)以及使用微波的生物医学传感中找到应用。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6e47/9626603/64388f8ab1a0/41598_2022_23119_Fig1_HTML.jpg

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