Shi Wenting, Liu Qing, Cao Jicheng, Dong Jianwei, Wang Zaifeng, Xu Min
School of Marine Science and Engineering, Nanjing Normal University, Nanjing 210023, People's Republic of China; Institute of Marine Science and Technology, Shandong University, Qingdao 266237, People's Republic of China.
School of Marine Science and Engineering, Nanjing Normal University, Nanjing 210023, People's Republic of China.
Mar Pollut Bull. 2023 Feb;187:114603. doi: 10.1016/j.marpolbul.2023.114603. Epub 2023 Jan 17.
In this study, we aimed to quantify the transport and fate of PAHs in different environmental phases (air, seawater, soil, sediment and fish), verify application of the Level III fugacity model in a bay simulation, and understand the transport and fate of PAHs in the bay environment on a macroscopic scale. The simulated average concentrations of ∑PAH in the air and soil (23.8 ng/m and 1080.91 ng/g, respectively), which is as a background reference data for the Haizhou Bay. In addition, the soil (307 t), fish (29.4 t), and sediment (9.72 t) phases were found to be important reservoirs in the Haizhou Bay. Emissions from road vehicles (658 t) accounted for the largest share of PAH emissions in the area, and atmospheric deposition contributed most to the input of PAHs to the polluted area in the region. Whereas the contribution of river runoff input was small, and degradation loss was the main output pathway.
在本研究中,我们旨在量化多环芳烃在不同环境相(空气、海水、土壤、沉积物和鱼类)中的迁移和归宿,验证三级逸度模型在海湾模拟中的应用,并从宏观尺度上了解多环芳烃在海湾环境中的迁移和归宿。模拟的空气中∑PAH平均浓度和土壤中∑PAH平均浓度分别为23.8 ng/m³和1080.91 ng/g,作为海州湾的背景参考数据。此外,发现土壤(307吨)、鱼类(29.4吨)和沉积物(9.72吨)相是海州湾中重要的储存库。道路车辆排放(658吨)占该地区多环芳烃排放的最大份额,大气沉降对该地区污染区域多环芳烃的输入贡献最大。而河流径流输入的贡献较小,降解损失是主要的输出途径。